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OODR-MPI SPECTROSCOPY OF AMMONIA INVOLVING A FAST PREDISSOCIATING INTERMEDIATE STATE
Jiang Bo; Xie Jichun; Sha Guohe; Xie Xinbing; Zhang Cunhao
刊名ACTA PHYSICO-CHIMICA SINICA
1989
DOI10.3866/PKU.WHXB19890309
5期:3页:293-298
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Chemistry, Physical
研究领域[WOS]Chemistry
英文摘要OOD-RMPI spectroscopy of ammonia using the fast predissociating (A) over bar state as the intermediate has proved to be a feasible approach to uncover hidden spectroscopic information on both the upper electronic states and the intermediate predissociating species. The rotationally resolved MPI spectra of NH3 and ND3 (X) over tilde -> (A) over bar (jv(2)) under bar -> (O) over bar' transition and correspondingly the rotational constants of ND3 C' (1)A(1)'(v(2) = 0,1) have been obtained. We found that only Q branch lines of NH3 (X) over tilde -> (A) over tilde 2-photon transition appeared when linearly polarised pumping light was used. At a series of different v(1) frequences, we can always get 2v(1)+v(2) resonant with a fixed (X) over tilde -> (C) over tilde revibronic transition line by tunning v(2). The intensity envelope of the ion signal thus obtained represents the rotational line profile of (A) over tilde state. From the width of the profile prodissociation life time of (A) over tilde is obtained.
语种英语
WOS记录号WOS:000207572200009
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文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/140965
专题中国科学院大连化学物理研究所
作者单位Acad Sinica, Dalian Inst Chem Phys, Dalian, Peoples R China
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Jiang Bo,Xie Jichun,Sha Guohe,et al. OODR-MPI SPECTROSCOPY OF AMMONIA INVOLVING A FAST PREDISSOCIATING INTERMEDIATE STATE[J]. ACTA PHYSICO-CHIMICA SINICA,1989,5(3):293-298.
APA Jiang Bo,Xie Jichun,Sha Guohe,Xie Xinbing,&Zhang Cunhao.(1989).OODR-MPI SPECTROSCOPY OF AMMONIA INVOLVING A FAST PREDISSOCIATING INTERMEDIATE STATE.ACTA PHYSICO-CHIMICA SINICA,5(3),293-298.
MLA Jiang Bo,et al."OODR-MPI SPECTROSCOPY OF AMMONIA INVOLVING A FAST PREDISSOCIATING INTERMEDIATE STATE".ACTA PHYSICO-CHIMICA SINICA 5.3(1989):293-298.
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