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题名: Direct spectroscopic observation of Fe(III)-phenolate complex formed from the reaction of benzene with peroxide species on Fe/ZSM-5 at room temperature
作者: Xia, Haian1;  Sun, Keqiang1;  Sun, Keju1;  Feng, Zhaochi1;  Li, Wei Xue1;  Li, Can1
刊名: JOURNAL OF PHYSICAL CHEMISTRY C
发表日期: 2008-06-19
DOI: 10.1021/jp800455x
卷: 112, 期:24, 页:9001-9005
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences ;  Technology
类目[WOS]: Chemistry, Physical ;  Nanoscience & Nanotechnology ;  Materials Science, Multidisciplinary
研究领域[WOS]: Chemistry ;  Science & Technology - Other Topics ;  Materials Science
英文摘要: The reaction of benzene with the active oxygen species was studied by UV-visible diffuse reflectance and Raman spectroscopies. For the first time, the intermediate Fe(III)-phenolate complex was evidenced by a UV-visible absorption band at 690 nm and the Raman bands at 643, 896, 990, 1149, 1228, 1475, 1580, and 1607 cm(-1). The Raman bands of the Fe(III)-phenolate complex were also confirmed by density functional theory calculations.
关键词[WOS]: NITROUS-OXIDE ;  N2O DECOMPOSITION ;  SELECTIVE OXIDATION ;  ACTIVE-SITES ;  MFI ZEOLITES ;  FEZSM-5 ZEOLITES ;  FE/MFI CATALYSTS ;  NOX REDUCTION ;  IRON ;  PHENOL
语种: 英语
WOS记录号: WOS:000256738900041
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/140974
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China

Recommended Citation:
Xia, Haian,Sun, Keqiang,Sun, Keju,et al. Direct spectroscopic observation of Fe(III)-phenolate complex formed from the reaction of benzene with peroxide species on Fe/ZSM-5 at room temperature[J]. JOURNAL OF PHYSICAL CHEMISTRY C,2008,112(24):9001-9005.
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