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题名: Organocatalytic Oxidative Dehydrogenation of Dihydroarenes by Dioxygen Using 2,3-Dichloro-5,6-dicyano-benzoquinone (DDQ) and NaNO2
作者: Zhang, Wei1, 2;  Ma, Hong1;  Zhou, Lipeng3;  Sun, Zhiqiang1;  Du, Zhongtian1;  Miao, Hong1;  Xu, Jie1
关键词: Oxidative dehydrogenation ;  DDQ ;  Dioxygen ;  Redox couples
刊名: MOLECULES
发表日期: 2008-12-01
DOI: 10.3390/molecules13123236
卷: 13, 期:12, 页:3236-3245
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Organic
研究领域[WOS]: Chemistry
英文摘要: The oxidative dehydrogenation of dihydroarenes catalyzed by 2,3-dichloro- 5,6-dicyano-benzoquinone(DDQ) and NaNO2 with dioxygen is reported. The combination of DDQ and NaNO2 showed high efficiency and high selectivity, compared with other benzoquinones and anthraquinones, e. g., >99% conversion of 9,10-dihydroanthracene with 99% selectivity for anthracene can be obtained at 120 degrees C under 1.3 MPa O-2 for 8 h. Excellent results were achieved in the oxidative dehydrogenation of variety of dihydroarenes.
关键词[WOS]: AEROBIC OXIDATION ;  MOLECULAR-OXYGEN ;  BENZYL ETHERS ;  EFFICIENT ;  HYDROCARBONS ;  AROMATIZATION ;  DEPROTECTION ;  CATALYSTS ;  QUINONES ;  ALCOHOLS
语种: 英语
WOS记录号: WOS:000261948300025
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/141043
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
2.Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China
3.Zhengzhou Univ, Dept Chem, Inst Catalysis, Zhengzhou 450001, Peoples R China

Recommended Citation:
Zhang, Wei,Ma, Hong,Zhou, Lipeng,et al. Organocatalytic Oxidative Dehydrogenation of Dihydroarenes by Dioxygen Using 2,3-Dichloro-5,6-dicyano-benzoquinone (DDQ) and NaNO2[J]. MOLECULES,2008,13(12):3236-3245.
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