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题名: Hydrogen storage capacity of nickel supported on a metal-organic framework compound under mild conditions
作者: Liu Yingya1, 2;  Zhang Jian1, 2;  Zeng Julan1, 2;  Chu Hailiang1, 2;  Xu Fen1;  Sun Lixian1
关键词: nickel ;  metal-organic framework compound ;  supported composite material ;  hydrogen storage capacity ;  impregnation ;  chemical reduction ;  hydrogen reduction
刊名: CHINESE JOURNAL OF CATALYSIS
发表日期: 2008-07-01
卷: 29, 期:7, 页:655-659
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences ;  Technology
类目[WOS]: Chemistry, Applied ;  Chemistry, Physical ;  Engineering, Chemical
研究领域[WOS]: Chemistry ;  Engineering
英文摘要: The traditional impregnation method was used to support nickel ions on the metal-organic framework compound MIL-101 (Cr(3)F(H(2)O)(2)O[(O(2)C)-C(6)H(4)-(CO(2))](3)center dot nH(2)O, n approximate to 5) for the preparation of a Ni/MIL-101 composite material. With two ways of impregnation (excessive impregnation and incipient wetness impregnation) followed by two ways of reduction (liquid chemical reduction and solid hydrogenation reduction), four Ni/MIL-101 samples were obtained. The hydrogen storage capacity of the Ni/MIL-101 samples was measured under mild conditions (25-100 degrees C, 0.01-4 MPa). Compared with the original MIL-101, Ni/MIL-101 had high hydrogen storage capacity because of the Ni particles supported on MIL-101. Among these samples, the sample prepared by excessive impregnation followed by liquid chemical reduction exhibited the highest hydrogen storage capacity of 1.02% at 100 degrees C and 4.0 MPa.
关键词[WOS]: HIGH H-2 ADSORPTION ;  COORDINATION POLYMER ;  SURFACE-AREA ;  INCLUSION ;  SPILLOVER ;  BINDING ;  MIL-101 ;  SITES ;  MOF ;  ZN
语种: 英语
WOS记录号: WOS:000258484400014
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/141190
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Liaoning, Peoples R China
2.Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China

Recommended Citation:
Liu Yingya,Zhang Jian,Zeng Julan,et al. Hydrogen storage capacity of nickel supported on a metal-organic framework compound under mild conditions[J]. CHINESE JOURNAL OF CATALYSIS,2008,29(7):655-659.
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