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Observation of the Interference between the Intramolecular IR-Visible and Visible-IR Processes in the Doubly Resonant Sum Frequency Generation Vibrational Spectroscopy of Rhodamine 6G Adsorbed at the Air/Water Interface
Wu, Dan; Deng, Gang-Hua; Guo, Yuan; Wang, Hong-fei1
刊名JOURNAL OF PHYSICAL CHEMISTRY A
2009-05-28
DOI10.1021/jp901655j
113期:21页:6058-6063
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Chemistry, Physical ; Physics, Atomic, Molecular & Chemical
研究领域[WOS]Chemistry ; Physics
关键词[WOS]LARGE ORGANIC-MOLECULES ; ELECTROCHEMICAL INTERFACE ; 2ND-HARMONIC GENERATION ; LIQUID INTERFACES ; XANTHENE DYES ; SURFACE ; PROBE ; RELAXATION ; SCATTERING ; METHYLENE
英文摘要Using the picosecond visible light at 532.1 nm and infrared light at 2800-3100 cm(-1), we observed the interference between the intramolecular IR-visible and visible-IR processes in the doubly resonant sum frequency generation vibrational spectroscopy of Rhodamine 6G adsorbed at the air/water interface. The interference phenomenon exists for both the C-H stretching vibrations in the 2800-3100 cm(-1) region and the skeleton vibrations in the 1450-1700 cm(-1) region. The relative strength of the visible-IR process at different wavelengths is the result of the electronic structure of the molecule. This is the first direct observation of the visible-IR sum frequency generation process in the electronically excited state of a model molecular system.
语种英语
WOS记录号WOS:000266296500004
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文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/141372
专题中国科学院大连化学物理研究所
作者单位1.Chinese Acad Sci, Beijing Natl Lab Mol Sci, Beijing 100190, Peoples R China
2.Chinese Acad Sci, State Key Lab Mol React Dynam, Inst Chem, Beijing 100190, Peoples R China
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Wu, Dan,Deng, Gang-Hua,Guo, Yuan,et al. Observation of the Interference between the Intramolecular IR-Visible and Visible-IR Processes in the Doubly Resonant Sum Frequency Generation Vibrational Spectroscopy of Rhodamine 6G Adsorbed at the Air/Water Interface[J]. JOURNAL OF PHYSICAL CHEMISTRY A,2009,113(21):6058-6063.
APA Wu, Dan,Deng, Gang-Hua,Guo, Yuan,&Wang, Hong-fei.(2009).Observation of the Interference between the Intramolecular IR-Visible and Visible-IR Processes in the Doubly Resonant Sum Frequency Generation Vibrational Spectroscopy of Rhodamine 6G Adsorbed at the Air/Water Interface.JOURNAL OF PHYSICAL CHEMISTRY A,113(21),6058-6063.
MLA Wu, Dan,et al."Observation of the Interference between the Intramolecular IR-Visible and Visible-IR Processes in the Doubly Resonant Sum Frequency Generation Vibrational Spectroscopy of Rhodamine 6G Adsorbed at the Air/Water Interface".JOURNAL OF PHYSICAL CHEMISTRY A 113.21(2009):6058-6063.
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