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题名: Preparation of Sulphonated Zirconium Phosphate-Phenylphosphonates and Their Catalytic Properties in Carbonylation of Formaldehyde
作者: Sun Ying1, 2;  Zhang Yangyang1;  Qi Yue1;  Wang Hua1;  Liu Hongchao1;  Shen Jianghan1;  Liu Zhongmin1
关键词: zirconium phenyl phosphonate ;  sulfonation ;  formaldehyde ;  carbonylation ;  methyl glycolate
刊名: CHINESE JOURNAL OF CATALYSIS
发表日期: 2009-08-01
卷: 30, 期:8, 页:786-790
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences ;  Technology
类目[WOS]: Chemistry, Applied ;  Chemistry, Physical ;  Engineering, Chemical
研究领域[WOS]: Chemistry ;  Engineering
英文摘要: Zirconium phenyl phosphonate Zr(C(6)H(5)PO(3))(2)center dot nH(2)O and its derivatives Zr(C(6)H(5)PO(3))(2)center dot(HPO(4))(x)center dot nH(2)O and Zr(C(6)H(5)PO(3))(2-x)(HPO(3))(x)center dot nH(2)O were synthesized and sulphonated. The pre- and post-sulfonation samples were characterized by inductively coupled plasma, X-ray diffraction, thermogravimetry, and infrared spectroscopy. The samples are all typical layered crystal with different interlayer spacings. Zirconium phosphate sulfophenylphosphonates (SZrPP-n) possessed high acidity amount and thermal stability. SZrPP-n was found to be an efficient and stable solid acid catalyst for carbonylation of formaldehyde.
关键词[WOS]: EXCHANGE RESIN CATALYSTS ;  METHYL METHOXY ACETATE ;  FORMATE ;  PHOSPHONATES ;  GLYCOLATE ;  SULFOPHOSPHONATES ;  HETEROPOLYACIDS ;  CONDENSATION ;  CHEMISTRY ;  AMINE
语种: 英语
WOS记录号: WOS:000270149200012
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/141421
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Liaoning, Peoples R China
2.Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China

Recommended Citation:
Sun Ying,Zhang Yangyang,Qi Yue,et al. Preparation of Sulphonated Zirconium Phosphate-Phenylphosphonates and Their Catalytic Properties in Carbonylation of Formaldehyde[J]. CHINESE JOURNAL OF CATALYSIS,2009,30(8):786-790.
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