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Oxidative Dehydrogenation of 9,10-Dihydroanthracene Catalyzed by 2,3-Dichloro-5,6-dicyano-1,4-benzoquinone/NaNO2
Zhang Wei1,2; Ma Hong1; Zhou Lipeng3; Miao Hong1; Xu Jie1
关键词Sodium Nitrite 2 3-dichloro-5 Oxidative Dehydrogenation 6-dicyano-1 9 4-benzoquinone 10-dihydroanthracene
刊名CHINESE JOURNAL OF CATALYSIS
2009-02-01
30期:2页:86-88
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Physical Sciences ; Technology
类目[WOS]Chemistry, Applied ; Chemistry, Physical ; Engineering, Chemical
研究领域[WOS]Chemistry ; Engineering
关键词[WOS]AEROBIC OXIDATION ; HYDROCARBONS ; OXYGENATION ; ALCOHOLS ; DIOXYGEN
英文摘要A catalyst for the oxidative dehydrogenation of 9, 10-dihydroanthracene to anthracene comprising 2,3-dichloro -5,6-dicyano-1,4-benzoquinone (DDQ) and NaNO2 showed high catalytic efficiency, with >99% conversion of 9, 10-dilaydroanthracene and 99% selectivity for anthracene at 120 degrees C under 1.3 MPa O-2 for 8 h. The reaction mechanism was investigated by FT-IR, H-1 NMR, and C-13 NMR. The two redox couples DDQ/DDQH(2) and NO2/NO were coupled in the presence of O-2 to create a catalytic cycle for the oxidative dehydrogenation of 9, 10-dihydroanthracene to anthracene.
语种英语
WOS记录号WOS:000264168700002
引用统计
被引频次:8[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/141583
专题中国科学院大连化学物理研究所
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
2.Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China
3.Zhengzhou Univ, Inst Catalysis, Dept Chem, Zhengzhou 450001, Henan, Peoples R China
推荐引用方式
GB/T 7714
Zhang Wei,Ma Hong,Zhou Lipeng,et al. Oxidative Dehydrogenation of 9,10-Dihydroanthracene Catalyzed by 2,3-Dichloro-5,6-dicyano-1,4-benzoquinone/NaNO2[J]. CHINESE JOURNAL OF CATALYSIS,2009,30(2):86-88.
APA Zhang Wei,Ma Hong,Zhou Lipeng,Miao Hong,&Xu Jie.(2009).Oxidative Dehydrogenation of 9,10-Dihydroanthracene Catalyzed by 2,3-Dichloro-5,6-dicyano-1,4-benzoquinone/NaNO2.CHINESE JOURNAL OF CATALYSIS,30(2),86-88.
MLA Zhang Wei,et al."Oxidative Dehydrogenation of 9,10-Dihydroanthracene Catalyzed by 2,3-Dichloro-5,6-dicyano-1,4-benzoquinone/NaNO2".CHINESE JOURNAL OF CATALYSIS 30.2(2009):86-88.
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