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题名: Aqueous hydrogenolysis of glycerol over Ni-Ce/AC catalyst: Promoting effect of Ce on catalytic performance
作者: Yu, Weiqiang1, 2;  Zhao, Jing1, 2;  Ma, Hong1;  Miao, Hong1;  Song, Qi1, 2;  Xu, Jie1
关键词: Aqueous hydrogenolysis ;  Cerium ;  Glycerol ;  Nickel
刊名: APPLIED CATALYSIS A-GENERAL
发表日期: 2010-07-31
DOI: 10.1016/j.apcata.2010.05.023
卷: 383, 期:1-2, 页:73-78
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences ;  Life Sciences & Biomedicine
类目[WOS]: Chemistry, Physical ;  Environmental Sciences
研究领域[WOS]: Chemistry ;  Environmental Sciences & Ecology
英文摘要: The aqueous hydrogenolysis of glycerol was performed over Ni-Ce/AC catalyst. The addition of cerium showed a remarkable promoting effect on the catalytic performance compared with other metals including copper, tin, zinc, aluminum, iron and cobalt. For example, 90.4% of glycerol conversion could be achieved at 473 K under 5 MPa of H(2) with 6 h. The Ni-Ce/AC catalysts were characterized by N(2) physisorption, XRD, TEM, NH(3)-TPD and H(2)-TPR. The results showed that the addition of cerium to the Ni/AC catalyst greatly changed the reductive behavior. (C) 2010 Elsevier B.V. All rights reserved.
关键词[WOS]: VAPOR-PHASE HYDROGENATION ;  AMORPHOUS ALLOY CATALYST ;  PROPYLENE-GLYCOL ;  SELECTIVE HYDROGENOLYSIS ;  NICKEL ;  CROTONALDEHYDE ;  CONVERSION ;  PHENOL ;  ACID
语种: 英语
WOS记录号: WOS:000280624900009
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/141688
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
2.Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China

Recommended Citation:
Yu, Weiqiang,Zhao, Jing,Ma, Hong,et al. Aqueous hydrogenolysis of glycerol over Ni-Ce/AC catalyst: Promoting effect of Ce on catalytic performance[J]. APPLIED CATALYSIS A-GENERAL,2010,383(1-2):73-78.
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