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Novel nickel-based catalyst for low temperature hydrogen production from methane steam reforming in membrane reformer
Chen, Yazhong1; Cui, Peng1; Xiong, Guoxing2; Xu, Hengyong2
关键词Hydrogen Production Membrane Reformer Methane Steam Reforming Novel Catalyst
刊名ASIA-PACIFIC JOURNAL OF CHEMICAL ENGINEERING
2010
DOI10.1002/apj.363
5期:1页:93-100
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Technology
类目[WOS]Engineering, Chemical
研究领域[WOS]Engineering
关键词[WOS]GLYCINE NITRATE PROCESS ; LIQUID HYDROCARBONS ; PARTIAL OXIDATION ; REACTOR ; SIMULATION ; FUELS
英文摘要Hydrogen production from various hydrocarbon fuels, particularly biomass-derived fuels, has attracted worldwide attention due to its potential for application to fuel cells, a device which converts chemical energy into electricity efficiently and cleanly. However, current technology, such as natural gas steam reforming, could not meet the specific requirements of hydrogen for fuel cells. Therefore, novel processes are intensively investigated, aiming to develop economic and efficient ones for the specific purpose. An important direction is the integrated membrane reformer for one-step high-purity hydrogen production. However, for the commercial realization of this technology, there are still some difficulties to overcome. By comparison with previous investigations with a similar membrane, this work showed that catalyst also played an important role in determining membrane reformer performance. We proposed that when thickness of membrane was several micrometers, the permeance of membrane became less important than the kinetics of catalyst, due to the fact that under Such conditions, hydrogen permeation rate was faster than the kinetics of steam reforming reaction when commercial catalyst was applied, but further evidence is indispensable. In this initial work, we focused on developing efficient nickel catalyst for low temperature steam reforming. Nickel-based catalyst was developed by deposition-coprecipitation and used as pre-reduced, showing high performance for methane steam reforming at low temperatures and good durability, which may find practical application for the integrated membrane reforming process. (C) 2009 Curtin University of Technology and John Wiley & Sons, Ltd.
语种英语
WOS记录号WOS:000275621800011
引用统计
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/141796
专题中国科学院大连化学物理研究所
作者单位1.Hefei Univ Technol, Sch Chem Engn, Hefei 230009, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
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GB/T 7714
Chen, Yazhong,Cui, Peng,Xiong, Guoxing,et al. Novel nickel-based catalyst for low temperature hydrogen production from methane steam reforming in membrane reformer[J]. ASIA-PACIFIC JOURNAL OF CHEMICAL ENGINEERING,2010,5(1):93-100.
APA Chen, Yazhong,Cui, Peng,Xiong, Guoxing,&Xu, Hengyong.(2010).Novel nickel-based catalyst for low temperature hydrogen production from methane steam reforming in membrane reformer.ASIA-PACIFIC JOURNAL OF CHEMICAL ENGINEERING,5(1),93-100.
MLA Chen, Yazhong,et al."Novel nickel-based catalyst for low temperature hydrogen production from methane steam reforming in membrane reformer".ASIA-PACIFIC JOURNAL OF CHEMICAL ENGINEERING 5.1(2010):93-100.
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