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Novel nickel-based catalyst for low temperature hydrogen production from methane steam reforming in membrane reformer
Chen, Yazhong1; Cui, Peng1; Xiong, Guoxing2; Xu, Hengyong2
KeywordHydrogen Production Membrane Reformer Methane Steam Reforming Novel Catalyst
Source PublicationASIA-PACIFIC JOURNAL OF CHEMICAL ENGINEERING
2010
DOI10.1002/apj.363
Volume5Issue:1Pages:93-100
Indexed BySCI
SubtypeArticle
WOS HeadingsScience & Technology ; Technology
WOS SubjectEngineering, Chemical
WOS Research AreaEngineering
WOS KeywordGLYCINE NITRATE PROCESS ; LIQUID HYDROCARBONS ; PARTIAL OXIDATION ; REACTOR ; SIMULATION ; FUELS
AbstractHydrogen production from various hydrocarbon fuels, particularly biomass-derived fuels, has attracted worldwide attention due to its potential for application to fuel cells, a device which converts chemical energy into electricity efficiently and cleanly. However, current technology, such as natural gas steam reforming, could not meet the specific requirements of hydrogen for fuel cells. Therefore, novel processes are intensively investigated, aiming to develop economic and efficient ones for the specific purpose. An important direction is the integrated membrane reformer for one-step high-purity hydrogen production. However, for the commercial realization of this technology, there are still some difficulties to overcome. By comparison with previous investigations with a similar membrane, this work showed that catalyst also played an important role in determining membrane reformer performance. We proposed that when thickness of membrane was several micrometers, the permeance of membrane became less important than the kinetics of catalyst, due to the fact that under Such conditions, hydrogen permeation rate was faster than the kinetics of steam reforming reaction when commercial catalyst was applied, but further evidence is indispensable. In this initial work, we focused on developing efficient nickel catalyst for low temperature steam reforming. Nickel-based catalyst was developed by deposition-coprecipitation and used as pre-reduced, showing high performance for methane steam reforming at low temperatures and good durability, which may find practical application for the integrated membrane reforming process. (C) 2009 Curtin University of Technology and John Wiley & Sons, Ltd.
Language英语
WOS IDWOS:000275621800011
Citation statistics
Cited Times:6[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/141796
Collection中国科学院大连化学物理研究所
Affiliation1.Hefei Univ Technol, Sch Chem Engn, Hefei 230009, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
Recommended Citation
GB/T 7714
Chen, Yazhong,Cui, Peng,Xiong, Guoxing,et al. Novel nickel-based catalyst for low temperature hydrogen production from methane steam reforming in membrane reformer[J]. ASIA-PACIFIC JOURNAL OF CHEMICAL ENGINEERING,2010,5(1):93-100.
APA Chen, Yazhong,Cui, Peng,Xiong, Guoxing,&Xu, Hengyong.(2010).Novel nickel-based catalyst for low temperature hydrogen production from methane steam reforming in membrane reformer.ASIA-PACIFIC JOURNAL OF CHEMICAL ENGINEERING,5(1),93-100.
MLA Chen, Yazhong,et al."Novel nickel-based catalyst for low temperature hydrogen production from methane steam reforming in membrane reformer".ASIA-PACIFIC JOURNAL OF CHEMICAL ENGINEERING 5.1(2010):93-100.
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