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题名: Transition-State Spectroscopy of Partial Wave Resonances in the F plus HD Reaction
作者: Dong, Wenrui1;  Xiao, Chunlei1;  Wang, Tao1;  Dai, Dongxu1;  Yang, Xueming1;  Zhang, Dong H.1
刊名: SCIENCE
发表日期: 2010-03-19
DOI: 10.1126/science.1185694
卷: 327, 期:5972, 页:1501-1502
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology
类目[WOS]: Multidisciplinary Sciences
研究领域[WOS]: Science & Technology - Other Topics
英文摘要: Partial wave resonances, quasi-bound resonance states with well-defined rotation in the transition state region of a chemical reaction, play a governing role in reaction dynamics but have eluded direct experimental characterization. Here, we report the observation of individual partial wave resolved resonances in the F + HD -> HF + D reaction by measuring the collision energy-dependent, angle-and state-resolved differential cross section with extremely high resolution, providing a spectroscopic probe to the transition state of F + HD -> HF + D. The agreement of the data with the high-level theoretical calculations confirms the sensitivity of this probe to the subtle quantum mechanical factors guiding this benchmark reaction.
关键词[WOS]: CHEMICAL-REACTION
语种: 英语
WOS记录号: WOS:000275715200045
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/141838
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Liaoning, Peoples R China

Recommended Citation:
Dong, Wenrui,Xiao, Chunlei,Wang, Tao,et al. Transition-State Spectroscopy of Partial Wave Resonances in the F plus HD Reaction[J]. SCIENCE,2010,327(5972):1501-1502.
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