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题名: Crossed molecular beam ion-imaging study of the Cl + SiH4 -> HCl + SiH3 reaction: product vibrational state-to-state correlation
作者: Wu, Guorong1;  Zhang, Weiqing1;  Pan, Huilin1;  Shuai, Quan1;  Yang, Jiayue1;  Jiang, Bo1;  Dai, Dongxu1;  Yang, Xueming1
刊名: PHYSICAL CHEMISTRY CHEMICAL PHYSICS
发表日期: 2010
DOI: 10.1039/b927455c
卷: 12, 期:32, 页:9469-9474
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Physical ;  Physics, Atomic, Molecular & Chemical
研究领域[WOS]: Chemistry ;  Physics
英文摘要: The dynamics of the Cl + SiH4 -> HCl + SiH3 reaction has been studied using the crossed molecular beam technique with slice imaging. The ion images of the silyl radical (SiH3) product from the Cl + SiH4 reaction were recorded at different collision energies, using the (2 + 1) resonance enhanced multi-photon ionization (REMPI) technique. The product velocity and angular distributions of this reaction were determined from the recorded images. The vibrational state-to-state correlation of the relative population between the two reaction products, SiH3 and HCl, was also determined. Finally, the Cl + SiH4 results are compared with that of the F + SiH4 reaction.
关键词[WOS]: ATOMIC CHLORINE ;  EXCITATION ;  DYNAMICS ;  METHANE ;  SILANE
语种: 英语
WOS记录号: WOS:000280708400042
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/141890
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Liaoning, Peoples R China

Recommended Citation:
Wu, Guorong,Zhang, Weiqing,Pan, Huilin,et al. Crossed molecular beam ion-imaging study of the Cl + SiH4 -> HCl + SiH3 reaction: product vibrational state-to-state correlation[J]. PHYSICAL CHEMISTRY CHEMICAL PHYSICS,2010,12(32):9469-9474.
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