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Crossed molecular beam ion-imaging study of the Cl + SiH4 -> HCl + SiH3 reaction: product vibrational state-to-state correlation
Wu, Guorong; Zhang, Weiqing; Pan, Huilin; Shuai, Quan; Yang, Jiayue; Jiang, Bo; Dai, Dongxu; Yang, Xueming
刊名PHYSICAL CHEMISTRY CHEMICAL PHYSICS
2010
DOI10.1039/b927455c
12期:32页:9469-9474
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Chemistry, Physical ; Physics, Atomic, Molecular & Chemical
研究领域[WOS]Chemistry ; Physics
关键词[WOS]ATOMIC CHLORINE ; EXCITATION ; DYNAMICS ; METHANE ; SILANE
英文摘要The dynamics of the Cl + SiH4 -> HCl + SiH3 reaction has been studied using the crossed molecular beam technique with slice imaging. The ion images of the silyl radical (SiH3) product from the Cl + SiH4 reaction were recorded at different collision energies, using the (2 + 1) resonance enhanced multi-photon ionization (REMPI) technique. The product velocity and angular distributions of this reaction were determined from the recorded images. The vibrational state-to-state correlation of the relative population between the two reaction products, SiH3 and HCl, was also determined. Finally, the Cl + SiH4 results are compared with that of the F + SiH4 reaction.
语种英语
WOS记录号WOS:000280708400042
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文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/141890
专题中国科学院大连化学物理研究所
作者单位Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Liaoning, Peoples R China
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Wu, Guorong,Zhang, Weiqing,Pan, Huilin,et al. Crossed molecular beam ion-imaging study of the Cl + SiH4 -> HCl + SiH3 reaction: product vibrational state-to-state correlation[J]. PHYSICAL CHEMISTRY CHEMICAL PHYSICS,2010,12(32):9469-9474.
APA Wu, Guorong.,Zhang, Weiqing.,Pan, Huilin.,Shuai, Quan.,Yang, Jiayue.,...&Yang, Xueming.(2010).Crossed molecular beam ion-imaging study of the Cl + SiH4 -> HCl + SiH3 reaction: product vibrational state-to-state correlation.PHYSICAL CHEMISTRY CHEMICAL PHYSICS,12(32),9469-9474.
MLA Wu, Guorong,et al."Crossed molecular beam ion-imaging study of the Cl + SiH4 -> HCl + SiH3 reaction: product vibrational state-to-state correlation".PHYSICAL CHEMISTRY CHEMICAL PHYSICS 12.32(2010):9469-9474.
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