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题名: Hydrogen production from ethanol steam reforming in a micro-channel reactor
作者: Cai, Weijie1;  Wang, Fagen1, 2;  van Veen, Andre1, 3;  Descorme, Claude1;  Schuurman, Yves1;  Shen, Wenjie2;  Mirodatos, Claude1
关键词: Hydrogen ;  Micro-reactor ;  Ethanol steam reforming ;  Iridium ;  Ceria
刊名: INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
发表日期: 2010-02-01
DOI: 10.1016/j.ijhydene.2009.11.104
卷: 35, 期:3, 页:1152-1159
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences ;  Technology
类目[WOS]: Chemistry, Physical ;  Electrochemistry ;  Energy & Fuels
研究领域[WOS]: Chemistry ;  Electrochemistry ;  Energy & Fuels
英文摘要: Ethanol steam reforming was studied over a supported Ir/CeO(2) catalyst in a micro-channel structured reactor. The catalyst coating was deposited on the channel walls and showed a remarkably high homogeneity and an excellent adherence to the stainless steel substrate, leading to stable performance during long-term runs. Hydrogen yields exceeding 40 L(H2) g(cat)(1) h(-1) were achieved during testing with partial ethanol conversion of 65% and a residence time in the order of a few milliseconds. This hydrogen productivity was found significantly higher than in a comparable conventional fixed-bed reactor hence being extremely promising for hydrogen production in micro fuel cell applications. (C) 2009 Professor T. Nejat Veziroglu. Published by Elsevier Ltd. All rights reserved.
关键词[WOS]: REACTION-MECHANISM ;  IR/CEO2 CATALYST ;  METAL-CATALYSTS ;  MICROREACTOR ;  OPTIMIZATION ;  PERFORMANCE ;  OXIDATION ;  SUPPORT ;  CO ;  PD
语种: 英语
WOS记录号: WOS:000274944000032
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/142012
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Univ Lyon 1, CNRS, IRCELYON, UMR 5256, F-69626 Villeurbanne, France
2.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
3.Ruhr Univ Bochum, Bochum, Germany

Recommended Citation:
Cai, Weijie,Wang, Fagen,van Veen, Andre,et al. Hydrogen production from ethanol steam reforming in a micro-channel reactor[J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,2010,35(3):1152-1159.
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