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题名: alpha,beta-Divinyl Tetrahydropyrroles as Chiral Chain Diene Ligands in Rhodium(l)-Catalyzed Enantioselective Conjugated Additions
作者: Li, Qian1;  Dong, Zhe1;  Yu, Zhi-Xiang1
刊名: ORGANIC LETTERS
发表日期: 2011-03-04
DOI: 10.1021/ol103152t
卷: 13, 期:5, 页:1122-1125
收录类别: SCI ;  IC ;  CCR
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Organic
研究领域[WOS]: Chemistry
英文摘要: A series of alpha,beta-divinyl tetrahydropyrroles, synthesized by asymmetric allylic C-H bond activation/conjugated diene addition reaction of ene-2-dienes, were found to be very efficient chiral chain diene ligands in the rhodium-catalyzed conjugated addition of organoboronic acids to various alpha,beta-unsaturated compounds, achieving the desired chiral adducts with good to excellent yields and ee values.
关键词[WOS]: CATALYZED ASYMMETRIC 1,4-ADDITION ;  ARYLBORONIC ACIDS ;  N-TOSYLARYLIMINES ;  STEERING LIGANDS ;  HIGH-PERFORMANCE ;  OLEFIN LIGANDS ;  BORONIC ACIDS ;  ARYLATION ;  COMPLEXES ;  TETRAFLUOROBENZOBARRELENES
语种: 英语
WOS记录号: WOS:000287645800078
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/142625
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Peking Univ, Coll Chem, Key Lab Bioorgan Chem & Mol Engn, Beijing Natl Lab Mol Sci BNLMS, Beijing 100871, Peoples R China

Recommended Citation:
Li, Qian,Dong, Zhe,Yu, Zhi-Xiang. alpha,beta-Divinyl Tetrahydropyrroles as Chiral Chain Diene Ligands in Rhodium(l)-Catalyzed Enantioselective Conjugated Additions[J]. ORGANIC LETTERS,2011,13(5):1122-1125.
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