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题名: Atomic and Molecular Clustering Kinetics in Gas Phase I. Basic Model of Chemical Kinetics
作者: Shi Yang1;  Gao Zhen1;  Zhu Qihe1;  Kong Fanao1
关键词: Cluster ;  Clustering kinetics ;  Size distribution of cluster
刊名: ACTA PHYSICO-CHIMICA SINICA
发表日期: 1996
DOI: 10.3866/PKU.WHXB19960302
卷: 12, 期:3, 页:196-201
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Physical
研究领域[WOS]: Chemistry
英文摘要: A general model is suggested for the kinetics of clustering processes. It is considered that cluster species are composed of units of specific composition. Arbitrary combinations occur between the species. The association rate constant depends on the cluster size and the structural feature. The dissociation rate constant mainly depend on the number of bonds broken during dissociation. Thus the small fragments are easier to be cleavaged. The master equations for the kinetic model are given. They can be used for the numercial calculation of the cluster distribution at various time. Finally, the clustering processes during laser ablation and are discharge are discussed.
语种: 英语
WOS记录号: WOS:000207599600002
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/142778
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Acad Sinica, Inst Chem, State Key Lab Mol React Dynam, Beijing 100080, Peoples R China

Recommended Citation:
Shi Yang,Gao Zhen,Zhu Qihe,et al. Atomic and Molecular Clustering Kinetics in Gas Phase I. Basic Model of Chemical Kinetics[J]. ACTA PHYSICO-CHIMICA SINICA,1996,12(3):196-201.
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