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Asymmetric Organocatalytic Cascade Michael/Michael/Henry Reaction Sequence: Control of All Stereocenters in One Cyclohexane Skeleton
Mao, Zhifeng1,2,3; Jia, Yaomei1,2; Xu, Zhaoqing3; Wang, Rui1,2
关键词Asymmetric Catalysis Cyclohexanes Domino Reactions Henry Reaction Michael Addition
刊名ADVANCED SYNTHESIS & CATALYSIS
2012-05-01
DOI10.1002/adsc.201200008
354期:8页:1401-1406
收录类别SCI ; IC ; CCR
文章类型Article
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Chemistry, Applied ; Chemistry, Organic
研究领域[WOS]Chemistry
关键词[WOS]DIPHENYLPROLINOL SILYL ETHER ; MICHAEL-HENRY REACTIONS ; HIGH-YIELDING SYNTHESIS ; FUNCTIONALIZED CYCLOHEXANES ; INHIBITOR (-)-OSELTAMIVIR ; CONTIGUOUS STEREOCENTERS ; BIFUNCTIONAL THIOUREA ; TANDEM REACTIONS ; BOND DONORS ; CATALYSIS
英文摘要The highly diastereo- and enantioselective relay cascade Michael/Michael/Henry reaction catalyzed by combination of readily available diphenylprolinol silyl ether and the quinine thiourea in a one-pot fashion has been developed. Up to 70% yield and up to >99% enantioselectivity of the single major isomer were obtained from the cascade reactions.
语种英语
WOS记录号WOS:000304345100003
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文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/142942
专题中国科学院大连化学物理研究所
作者单位1.Lanzhou Univ, Sch Basic Med Sci, Key Lab Preclin Study New Drugs Gansu Prov, Inst Biochem & Mol Biol,Sch Life Sci, Lanzhou 730000, Peoples R China
2.Lanzhou Univ, State Key Lab Appl Organ Chem, Lanzhou 730000, Peoples R China
3.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
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Mao, Zhifeng,Jia, Yaomei,Xu, Zhaoqing,et al. Asymmetric Organocatalytic Cascade Michael/Michael/Henry Reaction Sequence: Control of All Stereocenters in One Cyclohexane Skeleton[J]. ADVANCED SYNTHESIS & CATALYSIS,2012,354(8):1401-1406.
APA Mao, Zhifeng,Jia, Yaomei,Xu, Zhaoqing,&Wang, Rui.(2012).Asymmetric Organocatalytic Cascade Michael/Michael/Henry Reaction Sequence: Control of All Stereocenters in One Cyclohexane Skeleton.ADVANCED SYNTHESIS & CATALYSIS,354(8),1401-1406.
MLA Mao, Zhifeng,et al."Asymmetric Organocatalytic Cascade Michael/Michael/Henry Reaction Sequence: Control of All Stereocenters in One Cyclohexane Skeleton".ADVANCED SYNTHESIS & CATALYSIS 354.8(2012):1401-1406.
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