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题名: Hydrolysis reaction of ball-milled Mg-metal chlorides composite for hydrogen generation for fuel cells
作者: Wang, Shuang1, 3;  Sun, Li-Xian1, 4;  Xu, Fen2;  Jiao, Cheng-Li1, 3;  Zhang, Jian1;  Zhou, Huai-Ying4;  Huang, Feng-Lei5
关键词: Hydrogen generation ;  Mg-based-material ;  Ball milling ;  Hydrolysis reaction ;  Kinetics
刊名: INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
发表日期: 2012-04-01
DOI: 10.1016/j.ijhydene.2012.01.099
卷: 37, 期:8, 页:6771-6775
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences ;  Technology
类目[WOS]: Chemistry, Physical ;  Electrochemistry ;  Energy & Fuels
研究领域[WOS]: Chemistry ;  Electrochemistry ;  Energy & Fuels
英文摘要: In this paper, the hydrolysis properties for hydrogen generation by Mg-metal chlorides composites in pure water are investigated. The composites were prepared by high energy ball milling. It is found that the Mg-metal chlorides composites are very promising for hydrogen generation by hydrolysis reaction. The micro-galvanic cell formed by Mg and the other metal which produced by replacement reaction occurred during the ball-milling process is very effective for improving the hydrolysis reactivity. Based on the investigations of different kinds of chlorides additives, it is found that the Mg-10 wt% FeCl3 composite ball-milled for 30 min has the best hydrolysis properties with an initial hydrogen generation rate of 1479.1 ml*g(-1) min(-1) and a theoretical hydrogen production yield of 98% in 2 min. Copyright (C) 2012, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved.
关键词[WOS]: CHEMICAL HYDRIDES ;  MAGNESIUM ;  WATER
语种: 英语
WOS记录号: WOS:000303952300047
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/143026
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, Mat & Thermochem Lab, Dalian 116023, Peoples R China
2.Liaoning Normal Univ, Fac Chem & Chem Engn, Dalian 116029, Peoples R China
3.Chinese Acad Sci, Grad Sch, Beijing 100049, Peoples R China
4.Guilin Univ Elect Technol, Dept Mat Sci & Engn, Guilin 541004, Peoples R China
5.Beijing Inst Technol, State Key Lab Explos Sci & Technol, Beijing 100081, Peoples R China

Recommended Citation:
Wang, Shuang,Sun, Li-Xian,Xu, Fen,et al. Hydrolysis reaction of ball-milled Mg-metal chlorides composite for hydrogen generation for fuel cells[J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,2012,37(8):6771-6775.
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