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题名: Rh-III-Catalyzed Hydroacylation Reactions between N- Sulfonyl 2-Aminobenzaldehydes and Olefins
作者: Zhang, Tao1, 2;  Qi, Zisong1;  Zhang, Xueyun1;  Wu, Lamei2;  Li, Xingwei1
关键词: CH activation ;  cyclization ;  hydroacylation ;  olefins ;  rhodium
刊名: CHEMISTRY-A EUROPEAN JOURNAL
发表日期: 2014-03-17
DOI: 10.1002/chem.201400022
卷: 20, 期:12, 页:3283-3287
收录类别: SCI ;  IC ;  CCR
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Multidisciplinary
研究领域[WOS]: Chemistry
英文摘要: Metal-catalyzed hydroacylation of olefins represents an important atom-economic synthetic process in CH activation. For the first time highly efficient (RhCp)-Cp-III*-catalyzed hydroacylation was realized in the coupling of N-sulfonyl 2-aminobenzaldehydes with both conjugated and aliphatic olefins, leading to the synthesis of various aryl ketones. Occasionally, oxidative coupling occurred when a silver(I) oxidant was used.
关键词[WOS]: C-H BOND ;  INTERMOLECULAR HYDROACYLATION ;  OXIDATIVE OLEFINATION ;  DIRECTING GROUP ;  RHODIUM ;  ACTIVATION ;  CLEAVAGE ;  ALKYNES ;  SALICYLALDEHYDES ;  ALDEHYDES
语种: 英语
WOS记录号: WOS:000332747400005
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/143172
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
2.South Cent Univ Nationalities, Coll Chem & Mat Sci, Wuhan 430074, Peoples R China

Recommended Citation:
Zhang, Tao,Qi, Zisong,Zhang, Xueyun,et al. Rh-III-Catalyzed Hydroacylation Reactions between N- Sulfonyl 2-Aminobenzaldehydes and Olefins[J]. CHEMISTRY-A EUROPEAN JOURNAL,2014,20(12):3283-3287.
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