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学科主题: 物理化学
题名: Imine-linked conjugated organic polymer bearing bis(imino)pyridine ligands and its catalytic application in C-C coupling reactions
作者: Chen, Guifu1, 2;  Wang, Feng1;  Wang, Yehong1;  Zhang, Xiaochen1;  Qin, Hongqiang1;  Zou, Hanfa1;  Xu, Jie1
通讯作者: 王峰 ;  徐杰
关键词: Conjugated organic polymer material ;  Bis(imino)pyridine ligand ;  Catalysis ;  Suzuki-Miyaura C-C coupling
刊名: CHINESE JOURNAL OF CATALYSIS
发表日期: 2014-04-01
DOI: 10.1016/S1872-2067(14)60021-8
卷: 35, 期:4, 页:540-545
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences ;  Technology
类目[WOS]: Chemistry, Applied ;  Chemistry, Physical ;  Engineering, Chemical
研究领域[WOS]: Chemistry ;  Engineering
英文摘要: Covalent organic polymers are an emerging class of materials with potential applications in areas including molecular separation, gas sorption, and catalysis. A novel fully conjugated organic polymer bearing bis(imino)pyridine (COP-BIP) and its catalytic function are reported here. Unlike previous COP materials, the imine bonds of COP-BIP act as both linkages and complexation sites for the binding of metal ions. A clear structure is presented based on ultraviolet-visible, Fourier transform infrared, and matrix-assisted laser desorption/ionization time-of-flight mass spectrometry characterization. The COP-BIP materials are thermally stable up to 440 degrees C and are insoluble in conventional solvents. In addition, COP-BIP complexes Pd ions on bis(imino)pyridine sites and forms a heterogeneous catalyst, which exhibits excellent catalytic activity in the Suzuki-Miyaura C-C coupling reaction. 2014, Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. All rights reserved.
关键词[WOS]: FRAMEWORKS ;  COMPLEXES ;  HYDROGENATION
语种: 英语
WOS记录号: WOS:000333781700014
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/144107
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Liaoning, Peoples R China
2.Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China

Recommended Citation:
Chen, Guifu,Wang, Feng,Wang, Yehong,et al. Imine-linked conjugated organic polymer bearing bis(imino)pyridine ligands and its catalytic application in C-C coupling reactions[J]. CHINESE JOURNAL OF CATALYSIS,2014,35(4):540-545.
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