DICP OpenIR
Subject Area物理化学
One-pot catalytic conversion of cellulose to ethylene glycol and other chemicals: From fundamental discovery to potential commercialization
Zheng, Mingyuan; Pang, Jifeng; Wang, Aiqin; Zhang, Tao; Zhang T(张涛)
KeywordBiomass Cellulose Ethylene Glycol Tungstenic Catalyst Hydrogenation
Source PublicationCHINESE JOURNAL OF CATALYSIS
2014-05-01
DOI10.1016/S1872-2067(14)60013-9
Volume35Issue:5Pages:602-613
Indexed BySCI ; ISTP
SubtypeArticle
WOS HeadingsScience & Technology ; Physical Sciences ; Technology
WOS SubjectChemistry, Applied ; Chemistry, Physical ; Engineering, Chemical
WOS Research AreaChemistry ; Engineering
WOS KeywordTUNGSTEN CARBIDE CATALYSTS ; HYDRAZINE DECOMPOSITION ; LIGNOCELLULOSIC BIOMASS ; SELECTIVE CONVERSION ; BIMETALLIC CATALYSTS ; RANEY NI ; MICROCRYSTALLINE CELLULOSE ; 1,2-PROPYLENE GLYCOL ; GAMMA-VALEROLACTONE ; RUTHENIUM CATALYST
AbstractThe one-pot catalytic conversion of cellulose to ethylene glycol (CEG) is a highly attractive way for biomass utilization to lessen the consumption of fossil energy resources. In this paper, we reviewed the disclosure of the CEG process and the rapid progress in the development of highly efficient and robust catalysts for it. Based on our study of tungstenic catalysts, we discuss the reaction mechanism, in which the reaction routes, catalyst states, and catalytic roles of the tungsten species and hydrogenation sites in the cascade reactions are understood clearly. With future applications in mind, the conversion of raw cellulosic biomass and the strategy to develop an efficient CEG process for commercialization are discussed, and a model where the CEG process is incorporated into a bio-refinery process of acetone-n-butanol-ethanol (ABE) production is presented. (C) 2014, Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. All rights reserved.
Language英语
WOS IDWOS:000335622300002
Citation statistics
Cited Times:48[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/144217
Collection中国科学院大连化学物理研究所
Corresponding AuthorZhang T(张涛)
AffiliationChinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Liaoning, Peoples R China
Recommended Citation
GB/T 7714
Zheng, Mingyuan,Pang, Jifeng,Wang, Aiqin,et al. One-pot catalytic conversion of cellulose to ethylene glycol and other chemicals: From fundamental discovery to potential commercialization[J]. CHINESE JOURNAL OF CATALYSIS,2014,35(5):602-613.
APA Zheng, Mingyuan,Pang, Jifeng,Wang, Aiqin,Zhang, Tao,&张涛.(2014).One-pot catalytic conversion of cellulose to ethylene glycol and other chemicals: From fundamental discovery to potential commercialization.CHINESE JOURNAL OF CATALYSIS,35(5),602-613.
MLA Zheng, Mingyuan,et al."One-pot catalytic conversion of cellulose to ethylene glycol and other chemicals: From fundamental discovery to potential commercialization".CHINESE JOURNAL OF CATALYSIS 35.5(2014):602-613.
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