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Enhancement of Solar Hydrogen Evolution from Water by Surface Modification with CdS and TiO2 on Porous CuInS2 Photocathodes Prepared by an Electrodeposition-Sulfurization Method
Zhao, Jiao1,2,3; Minegishi, Tsutomu1; Zhang, Li1; Zhong, Miao2,4; Gunawan; Nakabayashi, Mamiko6; Ma, Guijun2,4; Hisatomi, Takashi1; Katayama, Masao1; Ikeda, Shigeru5; Shibata, Naoya6; Yamada, Taro4; Domen, Kazunari1
KeywordElectrodeposition Hydrogen Production I-iii-vi2 Chalcopyrites Photocathodes Photoelectrochemistry
Source PublicationANGEWANDTE CHEMIE-INTERNATIONAL EDITION
2014-10-27
DOI10.1002/anie.201406483
Volume53Issue:44Pages:11808-11812
Indexed BySCI
SubtypeArticle
WOS HeadingsScience & Technology ; Physical Sciences
WOS SubjectChemistry, Multidisciplinary
WOS Research AreaChemistry
WOS KeywordVISIBLE-LIGHT ; CELLS ; PHOTOABSORBER ; FABRICATION ; LAYERS
AbstractPorous films of p-type CuInS2, prepared by sulfurization of electrodeposited metals, are surface-modified with thin layers of CdS and TiO2. This specific porous electrode evolved H-2 from photoelectrochemical water reduction under simulated sunlight. Modification with thin n-type CdS and TiO2 layers significantly increased the cathodic photocurrent and onset potential through the formation of a p-n junction on the surface. The modified photocathodes showed a relatively high efficiency and stable H-2 production under the present reaction conditions.
Language英语
WOS IDWOS:000344050700015
Citation statistics
Cited Times:101[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/145443
Collection中国科学院大连化学物理研究所
Affiliation1.Univ Tokyo, Dept Chem Syst Engn, Bunkyo Ku, Tokyo 1138656, Japan
2.Artificial Photosynthet Chem Proc ARPChem, Japan Technol Res Assoc, Kashiwa, Chiba 2778589, Japan
3.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
4.Univ Tokyo, Dept Chem Syst Engn, Kashiwa, Chiba 2778589, Japan
5.Osaka Univ, Res Ctr Solar Energy Chem, Toyonaka, Osaka 5608531, Japan
6.Univ Tokyo, Inst Engn Innovat, Bunkyo Ku, Tokyo 1138656, Japan
Recommended Citation
GB/T 7714
Zhao, Jiao,Minegishi, Tsutomu,Zhang, Li,et al. Enhancement of Solar Hydrogen Evolution from Water by Surface Modification with CdS and TiO2 on Porous CuInS2 Photocathodes Prepared by an Electrodeposition-Sulfurization Method[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2014,53(44):11808-11812.
APA Zhao, Jiao.,Minegishi, Tsutomu.,Zhang, Li.,Zhong, Miao.,Gunawan.,...&Domen, Kazunari.(2014).Enhancement of Solar Hydrogen Evolution from Water by Surface Modification with CdS and TiO2 on Porous CuInS2 Photocathodes Prepared by an Electrodeposition-Sulfurization Method.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,53(44),11808-11812.
MLA Zhao, Jiao,et al."Enhancement of Solar Hydrogen Evolution from Water by Surface Modification with CdS and TiO2 on Porous CuInS2 Photocathodes Prepared by an Electrodeposition-Sulfurization Method".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 53.44(2014):11808-11812.
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