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题名: Enantioselective Copper-Catalyzed Decarboxylative Propargylic Alkylation of Propargylic Esters with beta-Keto Acids
作者: Zhu, Fu-Lin1, 2;  Wang, Ya-Hui1;  Zhang, De-Yang1, 2;  Hu, Xin-Hu1;  Chen, Song1;  Hou, Chuan-Jin1, 3;  Xu, Jie1;  Hu, Xiang-Ping1
关键词: asymmetric catalysis ;  copper ;  decarboxylative propargylic alkylation ;  beta-keto acids ;  propargylic esters
刊名: ADVANCED SYNTHESIS & CATALYSIS
发表日期: 2014-10-13
DOI: 10.1002/adsc.201400218
卷: 356, 期:14-15, 页:3231-3236
收录类别: SCI ;  CCR
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Applied ;  Chemistry, Organic
研究领域[WOS]: Chemistry
英文摘要: The first copper-catalyzed intermolecular enantioselective decarboxylative propargylic alkylation of propargylic esters with beta-keto acids as surrogates of ketones has been successfully developed by using a ketimine P, N, N-ligand. High yields and excellent enantioselectivities (up to 98% ee) have been achieved under the mild reaction conditions.
关键词[WOS]: SUBSTITUTION-REACTIONS ;  CONJUGATE ADDITION ;  1,3-DICARBONYL COMPOUNDS ;  3-HYDROXY OXINDOLES ;  TERMINAL ALKYNES ;  MANNICH REACTION ;  KETOACIDS ;  AMINATION ;  ACETATES ;  AMINES
语种: 英语
WOS记录号: WOS:000342906100043
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/145484
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Dalian Polytech Univ, Dalian 116034, Peoples R China

Recommended Citation:
Zhu, Fu-Lin,Wang, Ya-Hui,Zhang, De-Yang,et al. Enantioselective Copper-Catalyzed Decarboxylative Propargylic Alkylation of Propargylic Esters with beta-Keto Acids[J]. ADVANCED SYNTHESIS & CATALYSIS,2014,356(14-15):3231-3236.
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