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题名: Rh catalysts supported on knitting aryl network polymers for the hydroformylation of higher olefins
作者: Jiang, Miao1, 3;  Ding, Yunjie1, 2;  Yan, Li1;  Song, Xiangen1;  Lin, Ronghe1
关键词: Triphenylphosphine ;  Knitting aryl network polymer ;  Rhodium ;  Heterogeneous catalyst ;  Hydroformylation of higher olefins
刊名: CHINESE JOURNAL OF CATALYSIS
发表日期: 2014-09-01
DOI: 10.1016/S1872-2067(14)600684
卷: 35, 期:9, 页:1456-1464
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences ;  Technology
类目[WOS]: Chemistry, Applied ;  Chemistry, Physical ;  Engineering, Chemical
研究领域[WOS]: Chemistry ;  Engineering
英文摘要: Rh catalysts supported on knitting aryl network polymers (Rh/KAPs) were prepared for the hydroformylation of higher olefins. Rh catalysts supported on triphenylphosphine-benzene-base polymers (Rh/KAPs-1) showed higher activity for the higher olefins than Rh/SiO2 catalysts. Fourier transform infrared spectroscopy, thermogravimetry, N-2 adsorption-desorption, X-ray diffraction, transmission electron microscopy, C-13 NMR, and P-31 NMR showed that the Rh/ICAPs-1 catalysts have high thermal stability, high surface area, hierarchical porosity, highly dispersed Rh nanoparticles, and in situ formed homogeneous active species during the reaction. (C) 2014, Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. All rights reserved.
关键词[WOS]: MODIFIED RH/SIO2 CATALYST ;  CARBON-DIOXIDE CAPTURE ;  HETEROGENEOUS CATALYSTS ;  MICROPOROUS POLYMERS ;  MESOPOROUS SILICA ;  ORGANIC FRAMEWORK ;  NANOPARTICLES ;  WATER ;  HYDROGENATION ;  PROPYLENE
语种: 英语
WOS记录号: WOS:000341070700005
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/145566
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, Dalian 116023, Liaoning, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Liaoning, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China

Recommended Citation:
Jiang, Miao,Ding, Yunjie,Yan, Li,et al. Rh catalysts supported on knitting aryl network polymers for the hydroformylation of higher olefins[J]. CHINESE JOURNAL OF CATALYSIS,2014,35(9):1456-1464.
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