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题名: Effective thermodynamic alteration to Mg(NH2)(2)-LiH system: achieving near ambient-temperature hydrogen storage
作者: Cao, Hujun1, 2, 3;  Wu, Guotao1;  Zhang, Yao4;  Xiong, Zhitao1;  Qiu, Jieshan2;  Chen, Ping1
刊名: JOURNAL OF MATERIALS CHEMISTRY A
发表日期: 2014
DOI: 10.1039/c4ta03505d
卷: 2, 期:38, 页:15816-15822
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences ;  Technology
类目[WOS]: Chemistry, Physical ;  Energy & Fuels ;  Materials Science, Multidisciplinary
研究领域[WOS]: Chemistry ;  Energy & Fuels ;  Materials Science
英文摘要: A strategy for thermodynamic improvement of 2Mg(NH2)(2)-3LiH composite via "stabilizing" the dehydrogenated product LiNH2 was developed. By introducing LiI, LiBr and LiBH4 to the composite, hydrogen release at 0.1 MPa equilibrium pressure is thermodynamically allowed at 333, 320 and 337 K, respectively, which are ten degree Celsius lower than the pristine composite. Moreover, the dehydrogenation kinetics and reversibility are significantly improved.
关键词[WOS]: MG-N-H ;  COMPLEX HYDRIDES ;  AMIDE-HALIDE ;  LI4BN3H10 ;  IMIDES ;  LIBH4 ;  LIH ;  LINH2-MGH2 ;  RELEASE ;  LI3N
语种: 英语
WOS记录号: WOS:000342079200020
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/145579
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China
2.Dalian Univ Technol, Carbon Res Lab, Liaoning Key Lab Energy Mat & Chem Engn, State Key Lab Fine Chem, Dalian 116024, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
4.Southeast Univ, Sch Mat Sci & Engn, Nanjing 211189, Jiangsu, Peoples R China

Recommended Citation:
Cao, Hujun,Wu, Guotao,Zhang, Yao,et al. Effective thermodynamic alteration to Mg(NH2)(2)-LiH system: achieving near ambient-temperature hydrogen storage[J]. JOURNAL OF MATERIALS CHEMISTRY A,2014,2(38):15816-15822.
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