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Effective thermodynamic alteration to Mg(NH2)(2)-LiH system: achieving near ambient-temperature hydrogen storage
Cao, Hujun1,2,3; Wu, Guotao1; Zhang, Yao4; Xiong, Zhitao1; Qiu, Jieshan2; Chen, Ping1
刊名JOURNAL OF MATERIALS CHEMISTRY A
2014
DOI10.1039/c4ta03505d
2期:38页:15816-15822
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Physical Sciences ; Technology
类目[WOS]Chemistry, Physical ; Energy & Fuels ; Materials Science, Multidisciplinary
研究领域[WOS]Chemistry ; Energy & Fuels ; Materials Science
关键词[WOS]MG-N-H ; COMPLEX HYDRIDES ; AMIDE-HALIDE ; LI4BN3H10 ; IMIDES ; LIBH4 ; LIH ; LINH2-MGH2 ; RELEASE ; LI3N
英文摘要A strategy for thermodynamic improvement of 2Mg(NH2)(2)-3LiH composite via "stabilizing" the dehydrogenated product LiNH2 was developed. By introducing LiI, LiBr and LiBH4 to the composite, hydrogen release at 0.1 MPa equilibrium pressure is thermodynamically allowed at 333, 320 and 337 K, respectively, which are ten degree Celsius lower than the pristine composite. Moreover, the dehydrogenation kinetics and reversibility are significantly improved.
语种英语
WOS记录号WOS:000342079200020
引用统计
被引频次:21[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/145579
专题中国科学院大连化学物理研究所
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China
2.Dalian Univ Technol, Carbon Res Lab, Liaoning Key Lab Energy Mat & Chem Engn, State Key Lab Fine Chem, Dalian 116024, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
4.Southeast Univ, Sch Mat Sci & Engn, Nanjing 211189, Jiangsu, Peoples R China
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Cao, Hujun,Wu, Guotao,Zhang, Yao,et al. Effective thermodynamic alteration to Mg(NH2)(2)-LiH system: achieving near ambient-temperature hydrogen storage[J]. JOURNAL OF MATERIALS CHEMISTRY A,2014,2(38):15816-15822.
APA Cao, Hujun,Wu, Guotao,Zhang, Yao,Xiong, Zhitao,Qiu, Jieshan,&Chen, Ping.(2014).Effective thermodynamic alteration to Mg(NH2)(2)-LiH system: achieving near ambient-temperature hydrogen storage.JOURNAL OF MATERIALS CHEMISTRY A,2(38),15816-15822.
MLA Cao, Hujun,et al."Effective thermodynamic alteration to Mg(NH2)(2)-LiH system: achieving near ambient-temperature hydrogen storage".JOURNAL OF MATERIALS CHEMISTRY A 2.38(2014):15816-15822.
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