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题名: Rhodium-catalyzed tandem aldol condensation-Robinson annulation between aldehydes and acetone: synthesis of 3-methylcyclohexenones
作者: Wang, Fen1;  Liu, Yuchen1, 2;  Qi, Zisong1;  Dai, Wei2;  Li, Xingwei1
关键词: Rhodium catalysis ;  3-Methylcyclohexenones ;  Phenol ;  Robinson annulation
刊名: TETRAHEDRON LETTERS
发表日期: 2014-11-19
DOI: 10.1016/j.tetlet.2014.09.093
卷: 55, 期:47, 页:6399-6402
收录类别: SCI ;  IC ;  CCR
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Organic
研究领域[WOS]: Chemistry
英文摘要: A simple catalytic, redox-neutral access to 3-methylcyclohexenones has been developed via rhodium catalysis in the presence of an amine additive and Ag2CO3. This process utilized simple aldehydes and acetone as substrates and tolerates a variety of functional groups. Disubstituted phenols were isolated in moderate yields when Cu(OAc)(2) was employed as an oxidant. (C) 2014 Elsevier Ltd. All rights reserved.
关键词[WOS]: C-H ACTIVATION ;  ALPHA,BETA-UNSATURATED KETONES ;  AEROBIC DEHYDROGENATION ;  CYCLOHEXANONES ;  AROMATIZATION ;  ARYLATION ;  ARENES
语种: 英语
WOS记录号: WOS:000344825300003
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/145689
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
2.Zhejiang Normal Univ, Sch Chem & Biol Sci, Jinhua 321004, Peoples R China

Recommended Citation:
Wang, Fen,Liu, Yuchen,Qi, Zisong,et al. Rhodium-catalyzed tandem aldol condensation-Robinson annulation between aldehydes and acetone: synthesis of 3-methylcyclohexenones[J]. TETRAHEDRON LETTERS,2014,55(47):6399-6402.
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