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题名: Selective production of hydrogen peroxide and oxidation of hydrogen sulfide in an unbiased solar photoelectrochemical cell
作者: Zong, Xu1, 2, 3, 4;  Chen, Hongjun1, 2;  Seger, Brian5;  Pedersen, Thomas6;  Dargusch, Matthew S.7;  McFarland, Eric W.8;  Li, Can3, 4;  Wang, Lianzhou1, 2
刊名: ENERGY & ENVIRONMENTAL SCIENCE
发表日期: 2014-10-01
DOI: 10.1039/c4ee01503g
卷: 7, 期:10, 页:3347-3351
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences ;  Technology ;  Life Sciences & Biomedicine
类目[WOS]: Chemistry, Multidisciplinary ;  Energy & Fuels ;  Engineering, Chemical ;  Environmental Sciences
研究领域[WOS]: Chemistry ;  Energy & Fuels ;  Engineering ;  Environmental Sciences & Ecology
英文摘要: A solar-to-chemical conversion process is demonstrated using a photoelectrochemical cell without external bias for selective oxidation of hydrogen sulfide (H2S) to produce hydrogen peroxide (H2O2) and sulfur (S). The process integrates two redox couples anthraquinone/anthrahydroquinone and I-/I-3(-), and conceptually illustrates the remediation of a waste product for producing valuable chemicals.
关键词[WOS]: VISIBLE-LIGHT IRRADIATION ;  PHOTOCATALYTIC H-2 EVOLUTION ;  ENERGY-CONVERSION ;  WATER ;  TIO2 ;  SEMICONDUCTOR ;  GENERATION ;  CATALYSTS ;  DRIVEN ;  H2O2
语种: 英语
WOS记录号: WOS:000342884300018
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/145835
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Univ Queensland, Sch Chem Engn, Nanomat Ctr, Brisbane, Qld 4072, Australia
2.Univ Queensland, AIBN, Brisbane, Qld 4072, Australia
3.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
4.Dalian Lab Clean Energy, Dalian 116023, Peoples R China
5.Tech Univ Denmark, Dept Phys, CINF, DK-2800 Lyngby, Denmark
6.Tech Univ Denmark, Dept Micro & Nanotechnol, DK-2800 Lyngby, Denmark
7.Univ Queensland, Sch Mech & Min Engn, Ctr Adv Mat Proc & Mfg, Brisbane, Qld 4072, Australia
8.Univ Queensland, Sch Chem Engn, UQs Dow Ctr Sustainable Engn Innovat, Brisbane, Qld 4072, Australia

Recommended Citation:
Zong, Xu,Chen, Hongjun,Seger, Brian,et al. Selective production of hydrogen peroxide and oxidation of hydrogen sulfide in an unbiased solar photoelectrochemical cell[J]. ENERGY & ENVIRONMENTAL SCIENCE,2014,7(10):3347-3351.
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