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题名: Facile synthesis of POM@MOF embedded in SBA-15 as a steady catalyst for the hydroxylation of benzene
作者: Yang, Hua1;  Li, Jun1;  Zhang, Hengyun1;  Lv, Ying1;  Gao, Shuang1
关键词: MOF ;  Polyoxometallate ;  Hydroxylation ;  Catalysis ;  Hybrid mesoporous silica
刊名: MICROPOROUS AND MESOPOROUS MATERIALS
发表日期: 2014-09-01
DOI: 10.1016/j.micromeso.2014.04.023
卷: 195, 页:87-91
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences ;  Technology
类目[WOS]: Chemistry, Applied ;  Chemistry, Physical ;  Nanoscience & Nanotechnology ;  Materials Science, Multidisciplinary
研究领域[WOS]: Chemistry ;  Science & Technology - Other Topics ;  Materials Science
英文摘要: We present here a new hybrid material (POM@MOF@SBA-15, PMS) in which metal organic framework (MOF) MOF-199 encapsulated Kegginpolyoxometalate (POM) catalyst (names as POM@MOF) was facilely confined in mesoporous SBA-15. This mesoporous SBA-15 confined MOF-199 with encapsulated Keggin POM material was exploited to act as a stable heterogeneous POMs-based catalyst in a liquid oxidative reaction medium. Cycling experiments of the PMS catalyst were carried out in the direct synthesis of phenol from benzene and demonstrated unprecedented stability of this novel type PMS catalyst. (c) 2014 Elsevier Inc. All rights reserved.
关键词[WOS]: METAL-ORGANIC FRAMEWORK ;  DIBLOCK COPOLYMER ;  MULTILAYER FILMS ;  OXIDATION ;  SILICA ;  POLYOXOMETALATE ;  ACID ;  ESTERIFICATION ;  SEPARATION ;  VANADIUM
语种: 英语
WOS记录号: WOS:000337770900012
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/145844
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China

Recommended Citation:
Yang, Hua,Li, Jun,Zhang, Hengyun,et al. Facile synthesis of POM@MOF embedded in SBA-15 as a steady catalyst for the hydroxylation of benzene[J]. MICROPOROUS AND MESOPOROUS MATERIALS,2014,195:87-91.
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