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Facile synthesis of POM@MOF embedded in SBA-15 as a steady catalyst for the hydroxylation of benzene
Yang, Hua; Li, Jun; Zhang, Hengyun; Lv, Ying; Gao, Shuang
关键词Mof Polyoxometallate Hydroxylation Catalysis Hybrid Mesoporous Silica
刊名MICROPOROUS AND MESOPOROUS MATERIALS
2014-09-01
DOI10.1016/j.micromeso.2014.04.023
195页:87-91
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Physical Sciences ; Technology
类目[WOS]Chemistry, Applied ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
研究领域[WOS]Chemistry ; Science & Technology - Other Topics ; Materials Science
关键词[WOS]METAL-ORGANIC FRAMEWORK ; DIBLOCK COPOLYMER ; MULTILAYER FILMS ; OXIDATION ; SILICA ; POLYOXOMETALATE ; ACID ; ESTERIFICATION ; SEPARATION ; VANADIUM
英文摘要We present here a new hybrid material (POM@MOF@SBA-15, PMS) in which metal organic framework (MOF) MOF-199 encapsulated Kegginpolyoxometalate (POM) catalyst (names as POM@MOF) was facilely confined in mesoporous SBA-15. This mesoporous SBA-15 confined MOF-199 with encapsulated Keggin POM material was exploited to act as a stable heterogeneous POMs-based catalyst in a liquid oxidative reaction medium. Cycling experiments of the PMS catalyst were carried out in the direct synthesis of phenol from benzene and demonstrated unprecedented stability of this novel type PMS catalyst. (c) 2014 Elsevier Inc. All rights reserved.
语种英语
WOS记录号WOS:000337770900012
引用统计
被引频次:18[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/145844
专题中国科学院大连化学物理研究所
作者单位Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China
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GB/T 7714
Yang, Hua,Li, Jun,Zhang, Hengyun,et al. Facile synthesis of POM@MOF embedded in SBA-15 as a steady catalyst for the hydroxylation of benzene[J]. MICROPOROUS AND MESOPOROUS MATERIALS,2014,195:87-91.
APA Yang, Hua,Li, Jun,Zhang, Hengyun,Lv, Ying,&Gao, Shuang.(2014).Facile synthesis of POM@MOF embedded in SBA-15 as a steady catalyst for the hydroxylation of benzene.MICROPOROUS AND MESOPOROUS MATERIALS,195,87-91.
MLA Yang, Hua,et al."Facile synthesis of POM@MOF embedded in SBA-15 as a steady catalyst for the hydroxylation of benzene".MICROPOROUS AND MESOPOROUS MATERIALS 195(2014):87-91.
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