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Efficient aerobic oxidation of biomass-derived 5-hydroxymethylfurfural to 2,5-diformylfuran catalyzed by magnetic nanoparticle supported manganese oxide
Liu, Bing1,2; Zhang, Zehui1,2; Lv, Kangle1,2; Deng, Kejian1,2; Duan, Hongmin3
关键词Biomass Aerobic Oxidation 2 5-hydroxymethylfurfural 5-diformylfuran Manganese Oxide Magnetic Nanoparticles
刊名APPLIED CATALYSIS A-GENERAL
2014-02-22
DOI10.1016/j.apcata.2013.12.014
472页:64-71
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Physical Sciences ; Life Sciences & Biomedicine
类目[WOS]Chemistry, Physical ; Environmental Sciences
研究领域[WOS]Chemistry ; Environmental Sciences & Ecology
关键词[WOS]PULSED-LASER ABLATION ; HETEROGENEOUS CATALYST ; SELECTIVE OXIDATION ; IONIC LIQUIDS ; CONVERSION ; ACID ; DERIVATIVES ; CELLULOSE ; FRUCTOSE ; HEMICELLULOSE
英文摘要Magnetic Fe3O4 supported Mn3O4 nanoparticles (Fe3O4/Mn3O4) were prepared by the solvent thermal method, and its structure was characterized by XRD, XI'S, TEM, and FT-IR technologies. The resulting Fe3O4/Mn3O4 nanoparticles could be used as an excellent heterogeneous catalyst for the aerobic oxidation of the biomass-derived model molecule 5-hydroxymethylfurfural into 2,5-diformylfuran (DFF) under benign reaction conditions. Some important reaction parameters such as reaction temperature, catalyst amount, solvent, oxidant, and oxygen pressure were explored and high DFF yield of 82.1% with HMF conversion of 100% were obtained in DMF under optimal reaction conditions. More importantly, the catalyst could be readily separated from the reaction mixture by a permanent magnet, and recycled up to 6 times without the significant loss of its catalytic activity. (C) 2013 Elsevier B.V. All rights reserved.
语种英语
WOS记录号WOS:000333856200008
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被引频次:62[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/145875
专题中国科学院大连化学物理研究所
作者单位1.South Cent Univ Nationalities, Dept Chem, Key Lab Catalysis & Mat Sci, State Ethn Affairs Commiss, Wuhan 430074, Peoples R China
2.South Cent Univ Nationalities, Minist Educ, Wuhan 430074, Peoples R China
3.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China
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Liu, Bing,Zhang, Zehui,Lv, Kangle,et al. Efficient aerobic oxidation of biomass-derived 5-hydroxymethylfurfural to 2,5-diformylfuran catalyzed by magnetic nanoparticle supported manganese oxide[J]. APPLIED CATALYSIS A-GENERAL,2014,472:64-71.
APA Liu, Bing,Zhang, Zehui,Lv, Kangle,Deng, Kejian,&Duan, Hongmin.(2014).Efficient aerobic oxidation of biomass-derived 5-hydroxymethylfurfural to 2,5-diformylfuran catalyzed by magnetic nanoparticle supported manganese oxide.APPLIED CATALYSIS A-GENERAL,472,64-71.
MLA Liu, Bing,et al."Efficient aerobic oxidation of biomass-derived 5-hydroxymethylfurfural to 2,5-diformylfuran catalyzed by magnetic nanoparticle supported manganese oxide".APPLIED CATALYSIS A-GENERAL 472(2014):64-71.
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