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题名: Inorganic microporous membranes for H-2 and CO2 separation-Review of experimental and modeling progress
作者: Li, H.1;  Haas-Santo, K.2;  Schygulla, U.2;  Dittmeyer, R.2
关键词: Inorganic microporous membranes ;  Light gas separation ;  Performance ;  Hydrothermal stability ;  Over-all model
刊名: CHEMICAL ENGINEERING SCIENCE
发表日期: 2015-05-04
DOI: 10.1016/j.ces.2015.01.022
卷: 127, 页:401-417
收录类别: SCI
文章类型: Review
WOS标题词: Science & Technology ;  Technology
类目[WOS]: Engineering, Chemical
研究领域[WOS]: Engineering
英文摘要: Inorganic microporous membranes show great potential in several important applications, e.g., H-2 separation, the recovery of CO2 from natural gas and the reduction of green-house gas emission from flue gas. This article critically reviews latest progress in both experimental and modeling study of inorganic microporous membranes for relevant separation processes (i.e., H-2/CO2, CO2/N-2 and CO2/CH4 separation). Given significant improvement in gas separation performance as well as hydrothermal and chemical resilience, the evaluation of inorganic microporous membranes under industrial conditions is expected in the next step. The transport mechanisms and macroscopic models adopted for light gases are thoroughly discussed. An over-all model considering three relevant mechanisms, i.e., Knudsen diffusion (through defects), activated diffusion and surface diffusion, is highly desirable for the description of light gas transport. (C) 2015 Elsevier Ltd. All rights reserved.
关键词[WOS]: MOLECULAR-SIEVE MEMBRANES ;  METAL-ORGANIC FRAMEWORK ;  CARBON-DIOXIDE SEPARATION ;  CHEMICAL-VAPOR-DEPOSITION ;  GAS PERMEATION PROPERTIES ;  HOLLOW-FIBER MEMBRANES ;  MFI ZEOLITE MEMBRANES ;  MAXWELL-STEFAN DIFFUSIVITIES ;  SILICA MEMBRANES ;  HIGH-TEMPERATURE
语种: 英语
WOS记录号: WOS:000350860500037
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/146079
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China
2.Karlsruhe Inst Technol, Inst Micro Proc Engn IMVT, D-76344 Eggenstein Leopoldshafen, Germany

Recommended Citation:
Li, H.,Haas-Santo, K.,Schygulla, U.,et al. Inorganic microporous membranes for H-2 and CO2 separation-Review of experimental and modeling progress[J]. CHEMICAL ENGINEERING SCIENCE,2015,127:401-417.
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