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题名: Methanol to Olefins (MTO): From Fundamentals to Commercialization
作者: Tian, Peng1;  Wei, Yingxu1;  Ye, Mao1;  Liu, Zhongmin1, 2
关键词: methanol to olefins ;  DMTO ;  reaction mechanism ;  SAPO molecular sieve ;  scale-up ;  fluidized bed
刊名: ACS CATALYSIS
发表日期: 2015-03-01
DOI: 10.1021/acscatal.5b00007
卷: 5, 期:3, 页:1922-1938
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Physical
研究领域[WOS]: Chemistry
英文摘要: The methanol-to-olefins (MTO) reaction is an interesting and important reaction for both fundamental research and industrial application. The Dalian Institute of Chemical Physics (DICP) has developed a MTO technology that led to the successful construction and operation of the world's first coal to olefin plant in 2010. This historical perspective gives a brief summary on the key issues for the process development, including studies on the reaction mechanism, molecular sieve synthesis and crystallization mechanism, catalyst and its manufacturing scale up, reactor selection and reactor scale up, process demonstration, and commercialization. Further challenges on the fundamental research and the directions for future catalyst improvement are also suggested.
关键词[WOS]: SAPO MOLECULAR-SIEVES ;  TO-HYDROCARBONS REACTION ;  STATE NMR-SPECTROSCOPY ;  ACIDIC ZEOLITE CATALYSTS ;  RESEARCH-AND-DEVELOPMENT ;  FLUIDIZED-BED PROCESSES ;  IN-SITU NMR ;  REACTION-MECHANISM ;  COKE FORMATION ;  HEPTAMETHYLBENZENIUM CATION
语种: 英语
WOS记录号: WOS:000350843500059
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/146107
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, Natl Engn Lab Methanol Olefins, Dalian 116023, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China

Recommended Citation:
Tian, Peng,Wei, Yingxu,Ye, Mao,et al. Methanol to Olefins (MTO): From Fundamentals to Commercialization[J]. ACS CATALYSIS,2015,5(3):1922-1938.
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