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Layered Bi2Se3 Nanoplate/Polyvinylidene Fluoride Composite Based n-type Thermoelectric Fabrics
Dun, Chaochao1; Hewitt, Corey A.1; Huang, Huihui1,2; Xu, Junwei1; Montgomery, David S.1; Nie, Wanyi3; Jiang, Qike4; Carroll, David L.1
关键词Thermoelectric Layered Materials Flexible Bismuth Selenide Topological Insulator
刊名ACS APPLIED MATERIALS & INTERFACES
2015-04-08
DOI10.1021/acsami.5b00514
7期:13页:7054-7059
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Technology
类目[WOS]Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
研究领域[WOS]Science & Technology - Other Topics ; Materials Science
关键词[WOS]SINGLE DIRAC CONE ; CARBON NANOTUBES ; THERMOPOWER ; BI2TE3 ; FILMS ; POLY(3,4-ETHYLENEDIOXYTHIOPHENE) ; NANOCOMPOSITES ; PERFORMANCE ; BEHAVIOR ; SURFACE
英文摘要In this study, we report the fabrication of n-type flexible thermoelectric fabrics using layered Bi2Se3 nanoplate/polyvinylidene fluoride (PVDF) composites as the thermoelectric material. These composites exhibit room temperature Seebeck coefficient and electrical conductivity values of -80 mu V K-1 and 5100 S m(-1), respectively, resulting in a power factor approaching 30 mu W m(-1)K(-2). The temperature-dependent thermoelectric properties reveal that the composites exhibit metallic-like electrical conductivity, whereas the thermoelectric power is characterized by a heterogeneous model. These composites have the potential to be used in atypical applications for thermoelectrics, where lightweight and flexible materials would be beneficial. Indeed, bending tests revealed excellent durability of the thermoelectric fabrics. We anticipate that this work may guide the way for fabricating high performance thermoelectric fabrics based on layered V-VI nanoplates.
语种英语
WOS记录号WOS:000352751800002
引用统计
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/146170
专题中国科学院大连化学物理研究所
作者单位1.Wake Forest Univ, Dept Phys, Ctr Nanotechnol & Mol Mat, Winston Salem, NC 27109 USA
2.Shenzhen Univ, SZU NUS Collaborat Innovat Ctr Optoelect Sci & Te, Key Lab Optoelect Devices & Syst, Minist Educ & Guangdong Prov,Coll Optoelect Engn, Shenzhen 518060, Peoples R China
3.Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87544 USA
4.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
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Dun, Chaochao,Hewitt, Corey A.,Huang, Huihui,et al. Layered Bi2Se3 Nanoplate/Polyvinylidene Fluoride Composite Based n-type Thermoelectric Fabrics[J]. ACS APPLIED MATERIALS & INTERFACES,2015,7(13):7054-7059.
APA Dun, Chaochao.,Hewitt, Corey A..,Huang, Huihui.,Xu, Junwei.,Montgomery, David S..,...&Carroll, David L..(2015).Layered Bi2Se3 Nanoplate/Polyvinylidene Fluoride Composite Based n-type Thermoelectric Fabrics.ACS APPLIED MATERIALS & INTERFACES,7(13),7054-7059.
MLA Dun, Chaochao,et al."Layered Bi2Se3 Nanoplate/Polyvinylidene Fluoride Composite Based n-type Thermoelectric Fabrics".ACS APPLIED MATERIALS & INTERFACES 7.13(2015):7054-7059.
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