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Influence of Femtosecond Laser Parameters on Autler-Townes Splitting of Three-Level Ladder Molecules
Li, Yue-hua1; Lu, Xing-qiang2; Guo, Wei1; Yao, Hong-bin3
关键词Autler-townes Splitting Photoelectron Spectra Three-level Ladder K-2 Molecule
刊名CHINESE JOURNAL OF CHEMICAL PHYSICS
2015-04-01
DOI10.1063/1674-0068/28/cjcp1501006
28期:2页:128-133
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Physics, Atomic, Molecular & Chemical
研究领域[WOS]Physics
关键词[WOS]DRIVEN 4-LEVEL ATOMS ; SPONTANEOUS-EMISSION ; QUANTUM CONTROL ; FLUORESCENCE ; SPECTROSCOPY ; ABSORPTION ; SPECTRUM ; STATES ; FIELD ; K-2
英文摘要We theoretically investigate the Autler-Townes (AT) splitting in the photoelectron spectra of three-level ladder K-2 molecule driven by a pump-probe pulse via employing the time-dependent wave packet approach. The dependence of AT splitting on two laser intensities and wavelengths are studied in detail. We firstly quantify these effects on peak shift and AT separation. The photoelectron spectra show double splitting with symmetric profiles, but with asymmetric profiles when the wavelength is changed. The magnitude of AT splitting increases with the pump laser intensity, but does not vary with probe intensity. The shifts of the absorption peaks and the splitting between AT doublet are predicted by using an analytical fitting function when the intensity/wavelength of one of the two fields is changed. These novel results are of importance for the molecular spectroscopy and may further stimulate the first principles theoretical studies analytically.
语种英语
WOS记录号WOS:000354757300002
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文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/146248
专题中国科学院大连化学物理研究所
作者单位1.Univ South China, Sch Elect Engn, Hengyang 421001, Peoples R China
2.Univ South China, Sch Nucl Sci & Technol, Hengyang 421001, Peoples R China
3.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China
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Li, Yue-hua,Lu, Xing-qiang,Guo, Wei,et al. Influence of Femtosecond Laser Parameters on Autler-Townes Splitting of Three-Level Ladder Molecules[J]. CHINESE JOURNAL OF CHEMICAL PHYSICS,2015,28(2):128-133.
APA Li, Yue-hua,Lu, Xing-qiang,Guo, Wei,&Yao, Hong-bin.(2015).Influence of Femtosecond Laser Parameters on Autler-Townes Splitting of Three-Level Ladder Molecules.CHINESE JOURNAL OF CHEMICAL PHYSICS,28(2),128-133.
MLA Li, Yue-hua,et al."Influence of Femtosecond Laser Parameters on Autler-Townes Splitting of Three-Level Ladder Molecules".CHINESE JOURNAL OF CHEMICAL PHYSICS 28.2(2015):128-133.
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