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题名: Postfunctionalization of BN-Embedded Polycyclic Aromatic Compounds for Fine-Tuning of Their Molecular Properties
作者: Wang, Xiao-Ye1;  Yang, Dong-Chu1;  Zhuang, Fang-Dong1;  Liu, Jia-Jie1;  Wang, Jie-Yu1;  Pei, Jian1
关键词: boron ;  fluorescence ;  nitrogen ;  polycycles ;  synthesis design
刊名: CHEMISTRY-A EUROPEAN JOURNAL
发表日期: 2015-06-08
DOI: 10.1002/chem.201501161
卷: 21, 期:24, 页:8867-8873
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Multidisciplinary
研究领域[WOS]: Chemistry
英文摘要: New BN-embedded, thiophene-fused, polycyclic aromatic compounds with planar geometry were designed and synthesized. The molecules showed excellent stability and chemical robustness. Postfunctionalization on this skeleton was demonstrated with a series of electrophilic bromination, palladium-catalyzed cross-coupling, and Knoevenagel condensation reactions. The skeleton remained intact during these late-stage transformations. The optical and electronic properties have been well tuned through incorporation of electron-rich and -deficient groups on the backbone. This work shows the great advantage of the postfunctionalization strategy on BN-containing polycyclic aromatic compounds for fast diversification and materials screening.
关键词[WOS]: FIELD-EFFECT TRANSISTORS ;  ORGANIC SEMICONDUCTORS ;  CONJUGATED MATERIALS ;  PI-SYSTEMS ;  C-C ;  PERFORMANCE ;  HETEROACENES ;  POLYMERS ;  ANALOGS ;  DESIGN
语种: 英语
WOS记录号: WOS:000355287000031
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/146284
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Peking Univ, Key Lab Bioorgan Chem & Mol Engn, Ctr Soft Matter Sci & Engn, BNLMS,Minist Educ,Coll Chem & Mol Engn, Beijing 100871, Peoples R China

Recommended Citation:
Wang, Xiao-Ye,Yang, Dong-Chu,Zhuang, Fang-Dong,et al. Postfunctionalization of BN-Embedded Polycyclic Aromatic Compounds for Fine-Tuning of Their Molecular Properties[J]. CHEMISTRY-A EUROPEAN JOURNAL,2015,21(24):8867-8873.
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