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Postfunctionalization of BN-Embedded Polycyclic Aromatic Compounds for Fine-Tuning of Their Molecular Properties
Wang, Xiao-Ye; Yang, Dong-Chu; Zhuang, Fang-Dong; Liu, Jia-Jie; Wang, Jie-Yu; Pei, Jian
KeywordBoron Fluorescence Nitrogen Polycycles Synthesis Design
Source PublicationCHEMISTRY-A EUROPEAN JOURNAL
2015-06-08
DOI10.1002/chem.201501161
Volume21Issue:24Pages:8867-8873
Indexed BySCI
SubtypeArticle
WOS HeadingsScience & Technology ; Physical Sciences
WOS SubjectChemistry, Multidisciplinary
WOS Research AreaChemistry
WOS KeywordFIELD-EFFECT TRANSISTORS ; ORGANIC SEMICONDUCTORS ; CONJUGATED MATERIALS ; PI-SYSTEMS ; C-C ; PERFORMANCE ; HETEROACENES ; POLYMERS ; ANALOGS ; DESIGN
AbstractNew BN-embedded, thiophene-fused, polycyclic aromatic compounds with planar geometry were designed and synthesized. The molecules showed excellent stability and chemical robustness. Postfunctionalization on this skeleton was demonstrated with a series of electrophilic bromination, palladium-catalyzed cross-coupling, and Knoevenagel condensation reactions. The skeleton remained intact during these late-stage transformations. The optical and electronic properties have been well tuned through incorporation of electron-rich and -deficient groups on the backbone. This work shows the great advantage of the postfunctionalization strategy on BN-containing polycyclic aromatic compounds for fast diversification and materials screening.
Language英语
WOS IDWOS:000355287000031
Citation statistics
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/146284
Collection中国科学院大连化学物理研究所
AffiliationPeking Univ, Key Lab Bioorgan Chem & Mol Engn, Ctr Soft Matter Sci & Engn, BNLMS,Minist Educ,Coll Chem & Mol Engn, Beijing 100871, Peoples R China
Recommended Citation
GB/T 7714
Wang, Xiao-Ye,Yang, Dong-Chu,Zhuang, Fang-Dong,et al. Postfunctionalization of BN-Embedded Polycyclic Aromatic Compounds for Fine-Tuning of Their Molecular Properties[J]. CHEMISTRY-A EUROPEAN JOURNAL,2015,21(24):8867-8873.
APA Wang, Xiao-Ye,Yang, Dong-Chu,Zhuang, Fang-Dong,Liu, Jia-Jie,Wang, Jie-Yu,&Pei, Jian.(2015).Postfunctionalization of BN-Embedded Polycyclic Aromatic Compounds for Fine-Tuning of Their Molecular Properties.CHEMISTRY-A EUROPEAN JOURNAL,21(24),8867-8873.
MLA Wang, Xiao-Ye,et al."Postfunctionalization of BN-Embedded Polycyclic Aromatic Compounds for Fine-Tuning of Their Molecular Properties".CHEMISTRY-A EUROPEAN JOURNAL 21.24(2015):8867-8873.
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