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Visible/Infrared Dissociation of NO3: Roaming in the Dark or Roaming on the Ground?
Fernando, Ravin1; Dey, Arghya1; Broderick, Bernadette M.1; Fu, Bina2; Homayoon, Zahra3,4; Bowman, Joel M.3,4; Suits, Arthur G.1
刊名JOURNAL OF PHYSICAL CHEMISTRY A
2015-07-16
DOI10.1021/jp509902d
119期:28页:7163-7168
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Chemistry, Physical ; Physics, Atomic, Molecular & Chemical
研究领域[WOS]Chemistry ; Physics
关键词[WOS]POTENTIAL-ENERGY SURFACES ; PHOTODISSOCIATION DYNAMICS ; QUANTUM YIELDS ; PHOTOLYSIS ; CHANNELS ; DECOMPOSITION ; RADICALS ; STATES ; PATH
英文摘要We present a DC slice imaging study of roaming dynamics in the photodissociation of the nitrate radical, NO3, contrasting pure visible excitation with a combination of visible and CO2 laser excitation at 10.6 mu m. Images of specific rotational levels of NO are seen to reflect dissociation on the ground and first excited electronic states, as reported in previous work. The branching is obtained for specific rotational levels by comparison to quasiclassical trajectory calculations of the dynamics on these two surfaces. The results for the visible dissociation are found to be very similar to the combination of visible and infrared, raising questions about the nature of the coupling of these surfaces, the extent to which roaming takes place on both, and how the final product branching is determined.
语种英语
WOS记录号WOS:000358337600010
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被引频次:7[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/146437
专题中国科学院大连化学物理研究所
作者单位1.Wayne State Univ, Dept Chem, Detroit, MI 48202 USA
2.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China
3.Emory Univ, Dept Chem, Atlanta, GA 30322 USA
4.Emory Univ, Cherry L Emerson Ctr Sci Computat, Atlanta, GA 30322 USA
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Fernando, Ravin,Dey, Arghya,Broderick, Bernadette M.,et al. Visible/Infrared Dissociation of NO3: Roaming in the Dark or Roaming on the Ground?[J]. JOURNAL OF PHYSICAL CHEMISTRY A,2015,119(28):7163-7168.
APA Fernando, Ravin.,Dey, Arghya.,Broderick, Bernadette M..,Fu, Bina.,Homayoon, Zahra.,...&Suits, Arthur G..(2015).Visible/Infrared Dissociation of NO3: Roaming in the Dark or Roaming on the Ground?.JOURNAL OF PHYSICAL CHEMISTRY A,119(28),7163-7168.
MLA Fernando, Ravin,et al."Visible/Infrared Dissociation of NO3: Roaming in the Dark or Roaming on the Ground?".JOURNAL OF PHYSICAL CHEMISTRY A 119.28(2015):7163-7168.
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