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题名: A Career in Catalysis: Masatake Haruta
作者: Okumura, Mitsutaka1, 2;  Fujitani, Tadahiro3;  Huang, Jiahui4;  Ishida, Tamao5
关键词: gold nanoparticles ;  gold clusters ;  CO oxidation ;  propylene epoxidation ;  alcohol oxidation
刊名: ACS CATALYSIS
发表日期: 2015-08-01
DOI: 10.1021/acscatal.5b01122
卷: 5, 期:8, 页:4699-4707
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Physical
研究领域[WOS]: Chemistry
英文摘要: Professor Masatake Haruta's distinguished scientific achievements are highlighted in heterogeneous catalysis by gold (Au). In 1982, he discovered that Au became highly active for CO oxidation even at 200 K when gold was deposited as nanoparticles (NPs) smaller than 5 nm on 3d transition metal oxides. After this finding, he and his co-workers have developed many preparation methods for the deposition of Au as NPs and clusters onto a wide variety of supports. By kinetic, theoretical, and surface science studies, Haruta and co-workers revealed interesting catalytic features of Au, including reaction mechanisms which are greatly different from those of Pd and Pt. Haruta and co-workers also found that supported Au NPs catalyzed direct oxidation of propylene to propylene oxide using O-2 and H-2, and subsequently O-2 alone in the presence of H2O.
关键词[WOS]: SUPPORTED GOLD CATALYSTS ;  LOW-TEMPERATURE OXIDATION ;  VAPOR-PHASE EPOXIDATION ;  POROUS COORDINATION POLYMERS ;  CO OXIDATION ;  PROPYLENE EPOXIDATION ;  SELECTIVE OXIDATION ;  PROPENE EPOXIDATION ;  AEROBIC OXIDATION ;  GLUCOSE-OXIDATION
语种: 英语
WOS记录号: WOS:000359395100024
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/146453
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Osaka Univ, Grad Sch Sci, Dept Chem, Toyonaka, Osaka 5600043, Japan
2.Kyoto Univ, Elements Strategy Initiat Catalysts & Batteries, Kyoto 6158245, Japan
3.Natl Inst Adv Ind Sci & Technol, Interdisciplinary Res Ctr Catalyt Chem, Tsukuba, Ibaraki 3058565, Japan
4.Chinese Acad Sci, Gold Catalysis Res Ctr, State Key Lab Catalysis, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
5.Tokyo Metropolitan Univ, Res Ctr Gold Chem, Grad Sch Urban Environm Sci, Hachioji, Tokyo 1920397, Japan

Recommended Citation:
Okumura, Mitsutaka,Fujitani, Tadahiro,Huang, Jiahui,et al. A Career in Catalysis: Masatake Haruta[J]. ACS CATALYSIS,2015,5(8):4699-4707.
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