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题名: Hierarchically structured reactors containing nanocarbons for intensification of chemical reactions
作者: Garcia-Bordeje, Enrique1;  Liu, Yuefeng2, 3;  Su, Dang Sheng3;  Pham-Huu, Cuong2
刊名: JOURNAL OF MATERIALS CHEMISTRY A
发表日期: 2017-11-21
DOI: 10.1039/c7ta06826c
卷: 5, 期:43, 页:22408-22441
收录类别: SCI
文章类型: Review
WOS标题词: Science & Technology ;  Physical Sciences ;  Technology
类目[WOS]: Chemistry, Physical ;  Energy & Fuels ;  Materials Science, Multidisciplinary
研究领域[WOS]: Chemistry ;  Energy & Fuels ;  Materials Science
英文摘要: Carbon nanomaterials, such as carbon nanotubes, carbon nanofibers and graphene, featuring functional properties and tailored nanoscaEe dimensions have been widely used in different research fields, especially for catalysis and sustainable chemistry. Hierarchically structured reactors, combining nanoscopic coating carbon layers to disperse the active phase or even directly as metal-free catalysts, with controlled macroscopic shapes, have been extensively developed over the East few decades for numerous relevant catalytic processes, where mass and heat transfer is easily optimized for better catalytic performance and stability. The 3D structuration enables the full exploitation of the intrinsic activity of the catalyst and its industrial deployment without drawbacks [inked with nanomaterials. In this review article, we will summarize the recent developments involved in the field of hierarchically structured reactors, i.e. monoliths, foam and other materials, containing carbon nanomaterials. It is expected that such structured reactors will receive high scientific and industrial interest in the future not only in the field of catalysis but also in those [inked with wastewater purification or aerosol filtration processes. It will also be evidenced how hierarchically structured materials have contributed to the intensification of catalytic processes compared to conventional reactors, thus paving the way to the enhancement of other chemical reactions and their industrial deployment.
关键词[WOS]: ALIGNED CARBON NANOTUBES ;  METAL-FREE CATALYST ;  NANOFIBER/GRAPHITE-FELT COMPOSITE ;  FISCHER-TROPSCH SYNTHESIS ;  MODIFIED ACTIVATED CARBON ;  OXIDATIVE DEHYDROGENATION REACTIONS ;  SOLID FOAM PACKINGS ;  STAINLESS-STEEL ;  SILICON-CARBIDE ;  MASS-TRANSFER
语种: 英语
WOS记录号: WOS:000414605900001
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/149692
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.CSIC, Inst Carboquim, ICB, Miguel Luesma Castan 4, E-50018 Zaragoza, Spain
2.Univ Strasbourg, CNRS, Inst Chem & Proc Energy Environm & Hlth ICPEES, UMR 7515, 25 Rue Becquerel, F-67087 Strasbourg 08, France
3.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy DNL, 457 Zhongshan Rd, Dalian 116023, Peoples R China

Recommended Citation:
Garcia-Bordeje, Enrique,Liu, Yuefeng,Su, Dang Sheng,et al. Hierarchically structured reactors containing nanocarbons for intensification of chemical reactions[J]. JOURNAL OF MATERIALS CHEMISTRY A,2017,5(43):22408-22441.
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