DICP OpenIR
Robust Catalysis on 2D Materials Encapsulating Metals: Concept, Application, and Perspective
Deng, Jiao1,2; Deng, Dehui1,2; Bao, Xinhe1
Keyword2d Materials Chainmail For Catalyst Electron Penetration Graphene Nonprecious Metals
Source PublicationADVANCED MATERIALS
2017-11-20
DOI10.1002/adma.201606967
Volume29Issue:43
Indexed BySCI
SubtypeReview
WOS HeadingsScience & Technology ; Physical Sciences ; Technology
WOS SubjectChemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
WOS Research AreaChemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
WOS KeywordNITROGEN-DOPED CARBON ; OXYGEN REDUCTION REACTION ; HYDROGEN EVOLUTION REACTION ; SENSITIZED SOLAR-CELLS ; COUNTER ELECTRODE MATERIAL ; PERFORMANCE BIFUNCTIONAL ELECTROCATALYSTS ; HIGHLY EFFICIENT CATALYSIS ; IRON NANOPARTICLES ; ORGANIC FRAMEWORK ; CO NANOPARTICLES
AbstractGreat endeavors are undertaken to search for low-cost, rich-reserve, and highly efficient alternatives to replace precious-metal catalysts, in order to cut costs and improve the efficiency of catalysts in industry. However, one major problem in metal catalysts, especially nonprecious-metal catalysts, is their poor stability in real catalytic processes. Recently, a novel and promising strategy to construct 2D materials encapsulating nonprecious-metal catalysts has exhibited inimitable advantages toward catalysis, especially under harsh conditions (e.g., strong acidity or alkalinity, high temperature, and high overpotential). The concept, which originates from unique electron penetration through the 2D crystal layer from the encapsulated metals to promote a catalytic reaction on the outermost surface of the 2D crystal, has been widely applied in a variety of reactions under harsh conditions. It has been vividly described as "chainmail for catalyst." Herein, recent progress concerning this chainmail catalyst is reviewed, particularly focusing on the structural design and control with the associated electronic properties of such heterostructure catalysts, and also on their extensive applications in fuel cells, water splitting, CO2 conversion, solar cells, metal-air batteries, and heterogeneous catalysis. In addition, the current challenges that are faced in fundamental research and industrial application, and future opportunities for these fantastic catalytic materials are discussed.
Language英语
WOS IDWOS:000415142100001
Citation statistics
Cited Times:57[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/149723
Collection中国科学院大连化学物理研究所
Affiliation1.Chinese Acad Sci, Dalian Inst Chem Phys, Collaborat Innovat Ctr Chem Energy Mat iChEM, Dalian 116023, Peoples R China
2.Xiamen Univ, Coll Chem & Chem Engn, Collaborat Innovat Ctr Chem Energy Mat iChEM, State Key Lab Phys Chem Solid Surfaces, Xiamen 361005, Peoples R China
Recommended Citation
GB/T 7714
Deng, Jiao,Deng, Dehui,Bao, Xinhe. Robust Catalysis on 2D Materials Encapsulating Metals: Concept, Application, and Perspective[J]. ADVANCED MATERIALS,2017,29(43).
APA Deng, Jiao,Deng, Dehui,&Bao, Xinhe.(2017).Robust Catalysis on 2D Materials Encapsulating Metals: Concept, Application, and Perspective.ADVANCED MATERIALS,29(43).
MLA Deng, Jiao,et al."Robust Catalysis on 2D Materials Encapsulating Metals: Concept, Application, and Perspective".ADVANCED MATERIALS 29.43(2017).
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