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Exceptionally Active Assembled Dinuclear Ruthenium(II)-NNN Complex Catalysts for Transfer Hydrogenation of Ketones
Liu, Tingting1,2; Chai, Huining1,2; Wang, Liandi1; Yu, Zhengkun1,3
刊名ORGANOMETALLICS
2017-08-14
DOI10.1021/acs.organomet.7b00356
36期:15页:2914-2921
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Chemistry, Inorganic & Nuclear ; Chemistry, Organic
研究领域[WOS]Chemistry
关键词[WOS]ASYMMETRIC TRANSFER HYDROGENATION ; PYRAZOLYL-IMIDAZOLYL LIGAND ; HETEROMETALLIC COMPLEXES ; METAL-COMPLEXES ; NNN LIGAND ; BEARING ; OXIDATION ; OXYGEN ; WATER ; COOPERATIVITY
英文摘要Dinuclear ruthenium(II)-NNN complexes were efficiently assembled by means of coordinatively unsaturated 16-electron mononuclear ruthenium(II)-pyrazolyl-imidazolyl-pyridine complex and 4,4'-linked bipyridine ligands. The diruthenium(II)-NNN complex assembled through 4,4'-(CH2)(3)-bipyridine exhibited exceptionally high catalytic activity for the transfer hydrogenation (TH) of ketones in refluxing 2-propanol and reached TOF values up to 1.4 x 10(7) h(-1), demonstrating a remarkable cooperative effect from the ruthenium(II)-NNN functionalities.
语种英语
WOS记录号WOS:000407869100025
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文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/149821
专题中国科学院大连化学物理研究所
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, 457 Zhongshan Rd, Dalian 116023, Liaoning, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Chinese Acad Sci, Shanghai Inst Organ Chem, State Key Lab Organomet Chem, 354 Fenglin Rd, Shanghai 200032, Peoples R China
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Liu, Tingting,Chai, Huining,Wang, Liandi,et al. Exceptionally Active Assembled Dinuclear Ruthenium(II)-NNN Complex Catalysts for Transfer Hydrogenation of Ketones[J]. ORGANOMETALLICS,2017,36(15):2914-2921.
APA Liu, Tingting,Chai, Huining,Wang, Liandi,&Yu, Zhengkun.(2017).Exceptionally Active Assembled Dinuclear Ruthenium(II)-NNN Complex Catalysts for Transfer Hydrogenation of Ketones.ORGANOMETALLICS,36(15),2914-2921.
MLA Liu, Tingting,et al."Exceptionally Active Assembled Dinuclear Ruthenium(II)-NNN Complex Catalysts for Transfer Hydrogenation of Ketones".ORGANOMETALLICS 36.15(2017):2914-2921.
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