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Metal-Free Oxidation of Glycerol over Nitrogen-Containing Carbon Nanotubes
Gupta, Neeraj1; Khavryuchenko, Oleksiy2; Villa, Alberto3; Su, Dangsheng1,4
关键词Biomass Conversion Carbon Nanotubes Glycerol Metal-free Oxidation Ncnts
刊名CHEMSUSCHEM
2017-08-10
DOI10.1002/cssc.201700940
10期:15页:3030-3034
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Chemistry, Multidisciplinary
研究领域[WOS]Chemistry
关键词[WOS]SELECTIVE OXIDATION ; AEROBIC OXIDATION ; LIQUID-PHASE ; CATALYST ; NANOPARTICLES ; ALCOHOLS ; DIHYDROXYACETONE ; ACTIVATION ; CHEMICALS
英文摘要Nitrogen rich carbon nanotubes have been used as a metal free catalyst for the conversion of glycerol into dihydroxyacetone using tert-butyl hydroperoxide as an oxidant. Pyridine nitrogen groups embedded in a carbon matrix are identified as active sites for the reaction. Computational studies have demonstrated that oxidation of pyridine groups to pyridine oxime followed by hydrogen abstraction from secondary alcohol is likely responsible for the oxidation process.
语种英语
WOS记录号WOS:000407385500004
引用统计
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/149827
专题中国科学院大连化学物理研究所
作者单位1.Chinese Acad Sci, Catalysis Div, IMR Shenyang Natl Lab, Shenyang 110016, Liaoning, Peoples R China
2.TMM LLC, Res & Dev Dept, Volodymyrska Str 49a, Kiev, Ukraine
3.Univ Milan, Dipartimento Chim, Via Golgi 19, I-20133 Milan, Italy
4.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian, Peoples R China
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GB/T 7714
Gupta, Neeraj,Khavryuchenko, Oleksiy,Villa, Alberto,et al. Metal-Free Oxidation of Glycerol over Nitrogen-Containing Carbon Nanotubes[J]. CHEMSUSCHEM,2017,10(15):3030-3034.
APA Gupta, Neeraj,Khavryuchenko, Oleksiy,Villa, Alberto,&Su, Dangsheng.(2017).Metal-Free Oxidation of Glycerol over Nitrogen-Containing Carbon Nanotubes.CHEMSUSCHEM,10(15),3030-3034.
MLA Gupta, Neeraj,et al."Metal-Free Oxidation of Glycerol over Nitrogen-Containing Carbon Nanotubes".CHEMSUSCHEM 10.15(2017):3030-3034.
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