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题名: Metal-Free Oxidation of Glycerol over Nitrogen-Containing Carbon Nanotubes
作者: Gupta, Neeraj1;  Khavryuchenko, Oleksiy2;  Villa, Alberto3;  Su, Dangsheng1, 4
关键词: biomass conversion ;  carbon nanotubes ;  glycerol ;  metal-free oxidation ;  NCNTs
刊名: CHEMSUSCHEM
发表日期: 2017-08-10
DOI: 10.1002/cssc.201700940
卷: 10, 期:15, 页:3030-3034
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Multidisciplinary
研究领域[WOS]: Chemistry
英文摘要: Nitrogen rich carbon nanotubes have been used as a metal free catalyst for the conversion of glycerol into dihydroxyacetone using tert-butyl hydroperoxide as an oxidant. Pyridine nitrogen groups embedded in a carbon matrix are identified as active sites for the reaction. Computational studies have demonstrated that oxidation of pyridine groups to pyridine oxime followed by hydrogen abstraction from secondary alcohol is likely responsible for the oxidation process.
关键词[WOS]: SELECTIVE OXIDATION ;  AEROBIC OXIDATION ;  LIQUID-PHASE ;  CATALYST ;  NANOPARTICLES ;  ALCOHOLS ;  DIHYDROXYACETONE ;  ACTIVATION ;  CHEMICALS
语种: 英语
WOS记录号: WOS:000407385500004
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/149827
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Catalysis Div, IMR Shenyang Natl Lab, Shenyang 110016, Liaoning, Peoples R China
2.TMM LLC, Res & Dev Dept, Volodymyrska Str 49a, Kiev, Ukraine
3.Univ Milan, Dipartimento Chim, Via Golgi 19, I-20133 Milan, Italy
4.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian, Peoples R China

Recommended Citation:
Gupta, Neeraj,Khavryuchenko, Oleksiy,Villa, Alberto,et al. Metal-Free Oxidation of Glycerol over Nitrogen-Containing Carbon Nanotubes[J]. CHEMSUSCHEM,2017,10(15):3030-3034.
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