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Metal-Free Oxidation of Glycerol over Nitrogen-Containing Carbon Nanotubes
Gupta, Neeraj1; Khavryuchenko, Oleksiy2; Villa, Alberto3; Su, Dangsheng1,4
KeywordBiomass Conversion Carbon Nanotubes Glycerol Metal-free Oxidation Ncnts
Source PublicationCHEMSUSCHEM
2017-08-10
DOI10.1002/cssc.201700940
Volume10Issue:15Pages:3030-3034
Indexed BySCI
SubtypeArticle
WOS HeadingsScience & Technology ; Physical Sciences
WOS SubjectChemistry, Multidisciplinary
WOS Research AreaChemistry
WOS KeywordSELECTIVE OXIDATION ; AEROBIC OXIDATION ; LIQUID-PHASE ; CATALYST ; NANOPARTICLES ; ALCOHOLS ; DIHYDROXYACETONE ; ACTIVATION ; CHEMICALS
AbstractNitrogen rich carbon nanotubes have been used as a metal free catalyst for the conversion of glycerol into dihydroxyacetone using tert-butyl hydroperoxide as an oxidant. Pyridine nitrogen groups embedded in a carbon matrix are identified as active sites for the reaction. Computational studies have demonstrated that oxidation of pyridine groups to pyridine oxime followed by hydrogen abstraction from secondary alcohol is likely responsible for the oxidation process.
Language英语
WOS IDWOS:000407385500004
Citation statistics
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/149827
Collection中国科学院大连化学物理研究所
Affiliation1.Chinese Acad Sci, Catalysis Div, IMR Shenyang Natl Lab, Shenyang 110016, Liaoning, Peoples R China
2.TMM LLC, Res & Dev Dept, Volodymyrska Str 49a, Kiev, Ukraine
3.Univ Milan, Dipartimento Chim, Via Golgi 19, I-20133 Milan, Italy
4.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian, Peoples R China
Recommended Citation
GB/T 7714
Gupta, Neeraj,Khavryuchenko, Oleksiy,Villa, Alberto,et al. Metal-Free Oxidation of Glycerol over Nitrogen-Containing Carbon Nanotubes[J]. CHEMSUSCHEM,2017,10(15):3030-3034.
APA Gupta, Neeraj,Khavryuchenko, Oleksiy,Villa, Alberto,&Su, Dangsheng.(2017).Metal-Free Oxidation of Glycerol over Nitrogen-Containing Carbon Nanotubes.CHEMSUSCHEM,10(15),3030-3034.
MLA Gupta, Neeraj,et al."Metal-Free Oxidation of Glycerol over Nitrogen-Containing Carbon Nanotubes".CHEMSUSCHEM 10.15(2017):3030-3034.
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