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Visible light photocatalysis over solid acid: Enhanced by gold plasmonic effect
Lin, Feng1,2; Shao, Bin1; Li, Zhen3; Zhang, Junying1; Wang, Huan1; Zhang, Shaohua1; Haruta, Masatake1,4; Huang, Jiahui1
关键词Au Spr So42--tio2 Surface Acidity Pollutant Photocatalytic Oxidation
刊名APPLIED CATALYSIS B-ENVIRONMENTAL
2017-12-05
DOI10.1016/j.apcatb.2017.06.076
218页:480-487
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Physical Sciences ; Technology
类目[WOS]Chemistry, Physical ; Engineering, Environmental ; Engineering, Chemical
研究领域[WOS]Chemistry ; Engineering
关键词[WOS]HETEROGENEOUS PHOTOCATALYSIS ; CATALYTIC-OXIDATION ; HYDROGEN EVOLUTION ; DUAL COCATALYSTS ; SULFATED TIO2 ; PARTICLE-SIZE ; PHASE-CONTROL ; FERMI-LEVEL ; NANOPARTICLES ; THIOPHENE
英文摘要Solar driven catalysis by semiconductors is considered as a promising route to mitigate environmental problems caused by the combustion of fossil fuels and water pollution. Surface plasmon resonance (SPR) has offered a new opportunity to overcome the limited efficiency of photocatalysts. Herein we report that the SPR-mediated visible-light-responsive photocatalyst, 0.5 wt.% Au/SO42--TiO2, can achieve over 99% conversion of pollutants (thiophene, thiol, rhodamine B, and phenol) during photocatalytic oxidation with oxygen or air as oxidant under visible light irradiation. The considerable enhancement of photocatalytic activity can be attributed to the synergistic effect of Au SPR and Lewis acidic SO42--TiO2 which are beneficial for the efficient separation and transfer of the photo-generated electrons and holes. Such a strategy would be important to the design and preparation of highly photocatalytic active semiconductor catalysts. (C) 2017 Elsevier B.V. All rights reserved.
语种英语
WOS记录号WOS:000407983000046
引用统计
被引频次:4[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/149983
专题中国科学院大连化学物理研究所
作者单位1.Chinese Acad Sci, Gold Catalysis Res Ctr, State Key Lab Catalysis, Dalian Inst Chem Phys, 457 Zhongshan Rd, Dalian 116023, Peoples R China
2.Dalian Minzu Univ, Key Lab New Energy & Rare Earth Resource Utilizat, State Ethn Affairs Commiss, Sch Phys & Mat Engn, Dalian 116600, Peoples R China
3.Chinese Acad Sci, Dalian Natl Lab Clean Energy, Dalian Inst Chem Phys, 457 Zhongshan Rd, Dalian 116023, Peoples R China
4.Tokyo Metropolitan Univ, Res Ctr Gold Chem, Dept Appl Chem, Grad Sch Urban Environm Sci, 1-1 Minami Osawa, Hachioji, Tokyo 1920397, Japan
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Lin, Feng,Shao, Bin,Li, Zhen,et al. Visible light photocatalysis over solid acid: Enhanced by gold plasmonic effect[J]. APPLIED CATALYSIS B-ENVIRONMENTAL,2017,218:480-487.
APA Lin, Feng.,Shao, Bin.,Li, Zhen.,Zhang, Junying.,Wang, Huan.,...&Huang, Jiahui.(2017).Visible light photocatalysis over solid acid: Enhanced by gold plasmonic effect.APPLIED CATALYSIS B-ENVIRONMENTAL,218,480-487.
MLA Lin, Feng,et al."Visible light photocatalysis over solid acid: Enhanced by gold plasmonic effect".APPLIED CATALYSIS B-ENVIRONMENTAL 218(2017):480-487.
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