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题名: Synthesis of Diesel and Jet Fuel Range Alkanes with Furfural and Angelica Lactone
作者: Xu, Jilei1;  Li, Ning1, 2;  Yang, Xiaofeng1;  Li, Guangyi1;  Wang, Aiqin1, 2;  Cong, Yu1;  Wang, Xiaodong1;  Zhang, Tao1, 2
关键词: lignocellulose ;  diesel and jet fuels ;  angelica lactone ;  aldol condensation ;  hydrodeoxygenation
刊名: ACS CATALYSIS
发表日期: 2017-09-01
DOI: 10.1021/acscatal.7b01992
卷: 7, 期:9, 页:5880-5886
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Physical
研究领域[WOS]: Chemistry
英文摘要: A route was developed for the synthesis of diesel and jet fuel range C-9 and C-10 alkanes with furfural and angelica lactone, which can be obtained from hemicellulose and cellulose. It was found that angelica lactone is more reactive than levulinic acid or its other derivates in the aldol condensation with furfural. Among the investigated catalysts, Mn2O3 was found to be the most active and was very stable for the aldol condensation of furfural and angelica lactone. Over Mn2O3, a high carbon yield of C-10 oxygenates (about 96%) can be achieved by the aldol condensation of furfural and angelica lactone under mild conditions (353 K, 4 h). By the hydrogenation and hydrodeoxygenation of the aldol condensation product over the Pd/C and Pd-FeOx/SiO2 catalysts, high carbon yields (similar to 96%) of C-9 and C-10 alkanes were obtained.
关键词[WOS]: WOODY BIOMASS SOLIDS ;  HIGH-QUALITY DIESEL ;  GAMMA-VALEROLACTONE ;  CATALYTIC CONVERSION ;  LIGNOCELLULOSIC BIOMASS ;  TRANSPORTATION FUELS ;  BIMETALLIC CATALYSTS ;  ALDOL-CONDENSATION ;  LIQUID ALKANES ;  LEVULINIC ACID
语种: 英语
WOS记录号: WOS:000410005700036
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/150040
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, iChEM Collaborat Innovat Ctr Chem Energy Mat, Dalian 116023, Peoples R China

Recommended Citation:
Xu, Jilei,Li, Ning,Yang, Xiaofeng,et al. Synthesis of Diesel and Jet Fuel Range Alkanes with Furfural and Angelica Lactone[J]. ACS CATALYSIS,2017,7(9):5880-5886.
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