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Synthesis of Diesel and Jet Fuel Range Alkanes with Furfural and Angelica Lactone
Xu, Jilei1; Li, Ning1,2; Yang, Xiaofeng1; Li, Guangyi1; Wang, Aiqin1,2; Cong, Yu1; Wang, Xiaodong1; Zhang, Tao1,2
关键词Lignocellulose Diesel And Jet Fuels Angelica Lactone Aldol Condensation Hydrodeoxygenation
刊名ACS CATALYSIS
2017-09-01
DOI10.1021/acscatal.7b01992
7期:9页:5880-5886
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Chemistry, Physical
研究领域[WOS]Chemistry
关键词[WOS]WOODY BIOMASS SOLIDS ; HIGH-QUALITY DIESEL ; GAMMA-VALEROLACTONE ; CATALYTIC CONVERSION ; LIGNOCELLULOSIC BIOMASS ; TRANSPORTATION FUELS ; BIMETALLIC CATALYSTS ; ALDOL-CONDENSATION ; LIQUID ALKANES ; LEVULINIC ACID
英文摘要A route was developed for the synthesis of diesel and jet fuel range C-9 and C-10 alkanes with furfural and angelica lactone, which can be obtained from hemicellulose and cellulose. It was found that angelica lactone is more reactive than levulinic acid or its other derivates in the aldol condensation with furfural. Among the investigated catalysts, Mn2O3 was found to be the most active and was very stable for the aldol condensation of furfural and angelica lactone. Over Mn2O3, a high carbon yield of C-10 oxygenates (about 96%) can be achieved by the aldol condensation of furfural and angelica lactone under mild conditions (353 K, 4 h). By the hydrogenation and hydrodeoxygenation of the aldol condensation product over the Pd/C and Pd-FeOx/SiO2 catalysts, high carbon yields (similar to 96%) of C-9 and C-10 alkanes were obtained.
语种英语
WOS记录号WOS:000410005700036
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文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/150040
专题中国科学院大连化学物理研究所
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, iChEM Collaborat Innovat Ctr Chem Energy Mat, Dalian 116023, Peoples R China
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GB/T 7714
Xu, Jilei,Li, Ning,Yang, Xiaofeng,et al. Synthesis of Diesel and Jet Fuel Range Alkanes with Furfural and Angelica Lactone[J]. ACS CATALYSIS,2017,7(9):5880-5886.
APA Xu, Jilei.,Li, Ning.,Yang, Xiaofeng.,Li, Guangyi.,Wang, Aiqin.,...&Zhang, Tao.(2017).Synthesis of Diesel and Jet Fuel Range Alkanes with Furfural and Angelica Lactone.ACS CATALYSIS,7(9),5880-5886.
MLA Xu, Jilei,et al."Synthesis of Diesel and Jet Fuel Range Alkanes with Furfural and Angelica Lactone".ACS CATALYSIS 7.9(2017):5880-5886.
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