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Asymmetric Hydrogenation of Isoquinolines and Pyridines Using Hydrogen Halide Generated in Situ as Activator
Chen, Mu-Wang1; Ji, Yue1; Wang, Jie1; Chen, Qing-An1; Shi, Lei1; Zhou, Yong-Gui1,2
刊名ORGANIC LETTERS
2017-09-15
DOI10.1021/acs.orglett.7b02502
19期:18页:4988-4991
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Chemistry, Organic
研究领域[WOS]Chemistry
关键词[WOS]IRIDIUM-CATALYZED HYDROGENATION ; MULTIPLE STEREOGENIC CENTERS ; HALOGEN-BOND FORMATION ; ENANTIOSELECTIVE HYDROGENATION ; DIPHOSPHINE LIGANDS ; N-BROMOSUCCINIMIDE ; SALTS ; DERIVATIVES ; COMPLEXES ; BEARING
英文摘要By employing halogenide trichloroisocyanuric acid as a traceless activation reagent, a general iridium-catalyzed asymmetric hydrogenation of isoquinolines and pyridines is developed with up to 99% ee. This method avoids tedious steps of installation and removal of the activating groups. The mechanism studies indicated that hydrogen halide generated in situ acted as an activator of isoquinolines and pyridines.
语种英语
WOS记录号WOS:000411304300072
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文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/150066
专题中国科学院大连化学物理研究所
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
2.Chinese Acad Sci, Shanghai Inst Organ Chem, State Key Lab Organometall Chem, Shanghai 200032, Peoples R China
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GB/T 7714
Chen, Mu-Wang,Ji, Yue,Wang, Jie,et al. Asymmetric Hydrogenation of Isoquinolines and Pyridines Using Hydrogen Halide Generated in Situ as Activator[J]. ORGANIC LETTERS,2017,19(18):4988-4991.
APA Chen, Mu-Wang,Ji, Yue,Wang, Jie,Chen, Qing-An,Shi, Lei,&Zhou, Yong-Gui.(2017).Asymmetric Hydrogenation of Isoquinolines and Pyridines Using Hydrogen Halide Generated in Situ as Activator.ORGANIC LETTERS,19(18),4988-4991.
MLA Chen, Mu-Wang,et al."Asymmetric Hydrogenation of Isoquinolines and Pyridines Using Hydrogen Halide Generated in Situ as Activator".ORGANIC LETTERS 19.18(2017):4988-4991.
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