Chemistry, Applied
; Chemistry, Physical
; Engineering, Chemical
研究领域[WOS]:
Chemistry
; Engineering
英文摘要:
The idea that single metal atoms dispersed on a solid support can act as an efficient heterogeneous catalyst was raised in 2011 when single Pt atoms on an FeO, surface were reported to be active for CO oxidation and preferential oxidation of CO in Hz. The last six years have witnessed tremendous progress in the field of single-atom catalysis. Here we introduce the major achievements on this topic in 2015 and 2016. Some particular aspects of single-atom catalysis are discussed in depth, including new approaches in single-atom catalyst (SAC) synthesis, stable gold SACs for various reactions, the high selectivity of Pt and Pd SACs in hydrogenation, and the superior performance of non-noble metal SACs in electrochemistry. These accomplishments will encourage more efforts by researchers to achieve the controllable fabrication of SACs and explore their potential applications. (C) 2017, Dalian Institute of Chemical Physics, Chinese Academy of Sciences.
1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Liaoning, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
Recommended Citation:
Han, Bing,Lang, Rui,Qiao, Botao,et al. Highlights of the major progress in single-atom catalysis in 2015 and 2016[J]. CHINESE JOURNAL OF CATALYSIS,2017,38(9):1498-1507.