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Synthesis of Diesel and Jet Fuel Range Alkanes with Furfural and Angelica Lactone
Xu, Jilei1; Li, Ning1,2; Yang, Xiaofeng1; Li, Guangyi1; Wang, Aiqin1,2; Cong, Yu1; Wang, Xiaodong1; Zhang, Tao1,2
KeywordLignocellulose Diesel And Jet Fuels Angelica Lactone Aldol Condensation Hydrodeoxygenation
Source PublicationACS CATALYSIS
2017-09-01
DOI10.1021/acscatal.7b01992
Volume7Issue:9Pages:5880-5886
Indexed BySCI
SubtypeArticle
WOS HeadingsScience & Technology ; Physical Sciences
WOS SubjectChemistry, Physical
WOS Research AreaChemistry
WOS KeywordWOODY BIOMASS SOLIDS ; HIGH-QUALITY DIESEL ; GAMMA-VALEROLACTONE ; CATALYTIC CONVERSION ; LIGNOCELLULOSIC BIOMASS ; TRANSPORTATION FUELS ; BIMETALLIC CATALYSTS ; ALDOL-CONDENSATION ; LIQUID ALKANES ; LEVULINIC ACID
AbstractA route was developed for the synthesis of diesel and jet fuel range C-9 and C-10 alkanes with furfural and angelica lactone, which can be obtained from hemicellulose and cellulose. It was found that angelica lactone is more reactive than levulinic acid or its other derivates in the aldol condensation with furfural. Among the investigated catalysts, Mn2O3 was found to be the most active and was very stable for the aldol condensation of furfural and angelica lactone. Over Mn2O3, a high carbon yield of C-10 oxygenates (about 96%) can be achieved by the aldol condensation of furfural and angelica lactone under mild conditions (353 K, 4 h). By the hydrogenation and hydrodeoxygenation of the aldol condensation product over the Pd/C and Pd-FeOx/SiO2 catalysts, high carbon yields (similar to 96%) of C-9 and C-10 alkanes were obtained.
Language英语
WOS IDWOS:000410005700036
Citation statistics
Cited Times:9[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/150140
Collection中国科学院大连化学物理研究所
Affiliation1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, iChEM Collaborat Innovat Ctr Chem Energy Mat, Dalian 116023, Peoples R China
Recommended Citation
GB/T 7714
Xu, Jilei,Li, Ning,Yang, Xiaofeng,et al. Synthesis of Diesel and Jet Fuel Range Alkanes with Furfural and Angelica Lactone[J]. ACS CATALYSIS,2017,7(9):5880-5886.
APA Xu, Jilei.,Li, Ning.,Yang, Xiaofeng.,Li, Guangyi.,Wang, Aiqin.,...&Zhang, Tao.(2017).Synthesis of Diesel and Jet Fuel Range Alkanes with Furfural and Angelica Lactone.ACS CATALYSIS,7(9),5880-5886.
MLA Xu, Jilei,et al."Synthesis of Diesel and Jet Fuel Range Alkanes with Furfural and Angelica Lactone".ACS CATALYSIS 7.9(2017):5880-5886.
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