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题名: Electrochemical reduction of CO2 in solid oxide electrolysis cells
作者: Zhang, Lixiao1, 2;  Hu, Shiqing1, 2;  Zhu, Xuefeng1;  Yang, Weishen1
关键词: CO2 electrochemical reduction ;  SOECs ;  Ni-YSZ ;  MIECs
刊名: JOURNAL OF ENERGY CHEMISTRY
发表日期: 2017-07-01
DOI: 10.1016/j.jechem.2017.04.004
卷: 26, 期:4, 页:593-601
收录类别: SCI
文章类型: Review
WOS标题词: Science & Technology ;  Physical Sciences ;  Technology
类目[WOS]: Chemistry, Applied ;  Chemistry, Physical ;  Energy & Fuels ;  Engineering, Chemical
研究领域[WOS]: Chemistry ;  Energy & Fuels ;  Engineering
英文摘要: The effort on electrochemical reduction of CO2 to useful chemicals using the renewable energy to drive the process is growing fast recently. In this review, we introduce the recent progresses on the electrochemical reduction of CO2 in solid oxide electrolysis cells (SOECs). At high temperature, only CO is produced with high current densities and Faradic efficiency while the reactor is complicated and a better sealing technique is urgently needed. The typical electrolytes such as zirconia-based oxides, ceria-based oxides and lanthanum gallates-based oxides, anodes and cathodes are introduced in this review, and the cathode materials, such as conventional metal-ceramics (cermets), mixed ionic and electronic conductors (MIECs) are discussed in detail. In the future, to gain more value-added products, the electrolyte, cathode and anode materials should be developed to allow SOECs to be operated at temperature range of 573-873 K. At those temperatures, SOECs may combine the advantages of the low temperature system and the high temperature system to produce various products with high current densities. (C) 2017 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. and Science Press. All rights reserved.
关键词[WOS]: TEMPERATURE STEAM ELECTROLYSIS ;  CARBON-DIOXIDE ELECTROLYSIS ;  FUEL-CELLS ;  STABILIZED ZIRCONIA ;  IMPREGNATION METHODS ;  COMPOSITE ELECTRODE ;  IONIC-CONDUCTIVITY ;  OXYGEN DIFFUSION ;  ANODE MATERIALS ;  CATHODE
语种: 英语
WOS记录号: WOS:000412776100001
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/150179
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, State Key Lab Catalysis, Dalian Inst Chem Phys, Dalian 116023, Liaoning, Peoples R China
2.Univ Chinese Acad Sci, Dalian Inst Chem Phys, Beijing 100049, Peoples R China

Recommended Citation:
Zhang, Lixiao,Hu, Shiqing,Zhu, Xuefeng,et al. Electrochemical reduction of CO2 in solid oxide electrolysis cells[J]. JOURNAL OF ENERGY CHEMISTRY,2017,26(4):593-601.
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