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Electrochemical reduction of CO2 in solid oxide electrolysis cells
Zhang, Lixiao1,2; Hu, Shiqing1,2; Zhu, Xuefeng1; Yang, Weishen1
关键词Co2 Electrochemical Reduction Soecs Ni-ysz Miecs
刊名JOURNAL OF ENERGY CHEMISTRY
2017-07-01
DOI10.1016/j.jechem.2017.04.004
26期:4页:593-601
收录类别SCI
文章类型Review
WOS标题词Science & Technology ; Physical Sciences ; Technology
类目[WOS]Chemistry, Applied ; Chemistry, Physical ; Energy & Fuels ; Engineering, Chemical
研究领域[WOS]Chemistry ; Energy & Fuels ; Engineering
关键词[WOS]TEMPERATURE STEAM ELECTROLYSIS ; CARBON-DIOXIDE ELECTROLYSIS ; FUEL-CELLS ; STABILIZED ZIRCONIA ; IMPREGNATION METHODS ; COMPOSITE ELECTRODE ; IONIC-CONDUCTIVITY ; OXYGEN DIFFUSION ; ANODE MATERIALS ; CATHODE
英文摘要The effort on electrochemical reduction of CO2 to useful chemicals using the renewable energy to drive the process is growing fast recently. In this review, we introduce the recent progresses on the electrochemical reduction of CO2 in solid oxide electrolysis cells (SOECs). At high temperature, only CO is produced with high current densities and Faradic efficiency while the reactor is complicated and a better sealing technique is urgently needed. The typical electrolytes such as zirconia-based oxides, ceria-based oxides and lanthanum gallates-based oxides, anodes and cathodes are introduced in this review, and the cathode materials, such as conventional metal-ceramics (cermets), mixed ionic and electronic conductors (MIECs) are discussed in detail. In the future, to gain more value-added products, the electrolyte, cathode and anode materials should be developed to allow SOECs to be operated at temperature range of 573-873 K. At those temperatures, SOECs may combine the advantages of the low temperature system and the high temperature system to produce various products with high current densities. (C) 2017 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. and Science Press. All rights reserved.
语种英语
WOS记录号WOS:000412776100001
引用统计
被引频次:10[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/150179
专题中国科学院大连化学物理研究所
作者单位1.Chinese Acad Sci, State Key Lab Catalysis, Dalian Inst Chem Phys, Dalian 116023, Liaoning, Peoples R China
2.Univ Chinese Acad Sci, Dalian Inst Chem Phys, Beijing 100049, Peoples R China
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Zhang, Lixiao,Hu, Shiqing,Zhu, Xuefeng,et al. Electrochemical reduction of CO2 in solid oxide electrolysis cells[J]. JOURNAL OF ENERGY CHEMISTRY,2017,26(4):593-601.
APA Zhang, Lixiao,Hu, Shiqing,Zhu, Xuefeng,&Yang, Weishen.(2017).Electrochemical reduction of CO2 in solid oxide electrolysis cells.JOURNAL OF ENERGY CHEMISTRY,26(4),593-601.
MLA Zhang, Lixiao,et al."Electrochemical reduction of CO2 in solid oxide electrolysis cells".JOURNAL OF ENERGY CHEMISTRY 26.4(2017):593-601.
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