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Boosting CO2 electroreduction over layered zeolitic imidazolate frameworks decorated with Ag2O nanoparticles
Jiang, Xiaole1,2; Wu, Haihua1,2; Chang, Sujie3,4; Si, Rui5; Miao, Shu1; Huang, Weixin3,4; Li, Yanshuo3,4; Wang, Guoxiong1; Bao, Xinhe1
刊名JOURNAL OF MATERIALS CHEMISTRY A
2017-09-28
DOI10.1039/c7ta06114e
5期:36页:19371-19377
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Physical Sciences ; Technology
类目[WOS]Chemistry, Physical ; Energy & Fuels ; Materials Science, Multidisciplinary
研究领域[WOS]Chemistry ; Energy & Fuels ; Materials Science
关键词[WOS]ELECTROCHEMICAL REDUCTION ; CARBON-DIOXIDE ; ELECTRODES ; CATALYSIS ; OXIDE
英文摘要Silver (Ag) is one of the widely investigated catalysts for CO2 electroreduction. To improve the faradaic efficiency for CO production over Ag catalysts, many efforts have been devoted to tuning the size and morphology of Ag catalysts, using Ag-containing complex compounds or ionic liquid electrolyte. Herein, we report a strategy to enhance CO2 electroreduction by constructing a Ag2O/layered zeolitic imidazolate framework (ZIF) composite structure via one-pot hydrothermal treatment of ZIF-7 nanoparticles (NPs) in AgNO3 aqueous solution. The Ag2O/layered ZIF shows much higher CO faradaic efficiency and current density than the layered ZIF or Ag/C alone. The performance improvement in CO2 electroreduction over the Ag2O/layered ZIF is probably attributed to the synergistic effect between Ag2O NPs and the layered ZIF, as well as facilitated mass transport due to the high specific surface area of the Ag2O/layered ZIF.
语种英语
WOS记录号WOS:000411232100051
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文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/150188
专题中国科学院大连化学物理研究所
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, State Key Lab Catalysis,CAS Ctr Excellence Nanosc, Dalian 116023, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100039, Peoples R China
3.Univ Sci & Technol China, CAS Key Lab Mat Energy Convers, Hefei 230026, Anhui, Peoples R China
4.Univ Sci & Technol China, Dept Chem Phys, Hefei 230026, Anhui, Peoples R China
5.Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai Synchrotron Radiat Facil, Shanghai 201204, Peoples R China
6.Ningbo Univ, Sch Mat Sci & Chem Engn, Ningbo 315211, Zhejiang, Peoples R China
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Jiang, Xiaole,Wu, Haihua,Chang, Sujie,et al. Boosting CO2 electroreduction over layered zeolitic imidazolate frameworks decorated with Ag2O nanoparticles[J]. JOURNAL OF MATERIALS CHEMISTRY A,2017,5(36):19371-19377.
APA Jiang, Xiaole.,Wu, Haihua.,Chang, Sujie.,Si, Rui.,Miao, Shu.,...&Bao, Xinhe.(2017).Boosting CO2 electroreduction over layered zeolitic imidazolate frameworks decorated with Ag2O nanoparticles.JOURNAL OF MATERIALS CHEMISTRY A,5(36),19371-19377.
MLA Jiang, Xiaole,et al."Boosting CO2 electroreduction over layered zeolitic imidazolate frameworks decorated with Ag2O nanoparticles".JOURNAL OF MATERIALS CHEMISTRY A 5.36(2017):19371-19377.
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