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Macroscopic Wires from Fluorophore-Quencher Dyads with Long-Lived Blue Emission
Wang, Tao1,2; Wu, Ziye2; Sun, Wei1,2; Jin, Shengye3; Zhang, Xingyuan1; Zhou, Chuanyao3; Jiang, Jun1,2; Luo, Yi1,2; Zhang, Guoqing2
Source PublicationJOURNAL OF PHYSICAL CHEMISTRY A
2017-09-28
DOI10.1021/acs.jpca.7b08268
Volume121Issue:38Pages:7183-7190
Indexed BySCI
SubtypeArticle
WOS HeadingsScience & Technology ; Physical Sciences
WOS SubjectChemistry, Physical ; Physics, Atomic, Molecular & Chemical
WOS Research AreaChemistry ; Physics
WOS KeywordAGGREGATION-INDUCED EMISSION ; ACTIVATED DELAYED FLUORESCENCE ; LIGHT-EMITTING-DIODES ; ROOM-TEMPERATURE ; ENERGY-TRANSFER ; SINGLET-STATE ; TRIPLET ; CONVERSION ; OLEDS
AbstractWe report the formation of macroscopic wires up to centimeters in length from a series of structurally flexible, covalently tethered small-molecular fluorophore-quencher dyads (FQDs, average MW = 425 Da), comprised of carbazole, melatonin, and cyanobenzoate moieties. These FQDs are nonemissive in organic solutions but become moderately to highly luminescent (Phi(F) = 0.037-0.39) upon formation of wires with emission maxima in the blue region (446-483 nm). The blue photoluminescence (PL) is ascribed to a combination of singlet charge transfer, localized triplet state, and possibly delayed fluorescence emissions with intrinsic luminescence lifetimes ranging from 0.228 to 21333 mu s, based on luminescence, transient absorption measurements, X-ray diffraction, and calculations.
Language英语
WOS IDWOS:000412149600014
Citation statistics
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/150192
Collection中国科学院大连化学物理研究所
Affiliation1.Univ Sci & Technol China, Sch Chem & Mat Sci, Hefei 230026, Anhui, Peoples R China
2.Univ Sci & Technol China, Hefei Natl Lab Phys Sci Micro Scale, Hefei 230026, Anhui, Peoples R China
3.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China
Recommended Citation
GB/T 7714
Wang, Tao,Wu, Ziye,Sun, Wei,et al. Macroscopic Wires from Fluorophore-Quencher Dyads with Long-Lived Blue Emission[J]. JOURNAL OF PHYSICAL CHEMISTRY A,2017,121(38):7183-7190.
APA Wang, Tao.,Wu, Ziye.,Sun, Wei.,Jin, Shengye.,Zhang, Xingyuan.,...&Zhang, Guoqing.(2017).Macroscopic Wires from Fluorophore-Quencher Dyads with Long-Lived Blue Emission.JOURNAL OF PHYSICAL CHEMISTRY A,121(38),7183-7190.
MLA Wang, Tao,et al."Macroscopic Wires from Fluorophore-Quencher Dyads with Long-Lived Blue Emission".JOURNAL OF PHYSICAL CHEMISTRY A 121.38(2017):7183-7190.
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