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题名: Cobalt(III)- and Rhodium(III)-Catalyzed C-H Amidation and Synthesis of 4-Quinolones: C-H Activation Assisted by Weakly Coordinating and Functionalizable Enaminone
作者: Wang, Fen1, 3;  Jin, Liang1, 2;  Kong, Lingheng1;  Li, Xingwei1
刊名: ORGANIC LETTERS
发表日期: 2017-04-07
DOI: 10.1021/acs.orglett.7b00583
卷: 19, 期:7, 页:1812-1815
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Organic
研究领域[WOS]: Chemistry
英文摘要: Cobalt(III) and rhodiurn(III) catalysts exhibited complementary scope in C-H amidation of aryl enaminones. The amidation reactions proceeded with broad scope under the assistance of a weakly coordinating and bifunctional enaminone directing group. The electrophilicity of the enaminone group can be further utilized in subsequent hydrolysis-cyclization reactions to afford NH 4-quinolones in telescoping reactions.
关键词[WOS]: N BOND FORMATION ;  CARBON-NITROGEN BONDS ;  ROOM-TEMPERATURE ;  NATURAL-PRODUCTS ;  AMIDO TRANSFER ;  AMINATION ;  ARENES ;  AZIDES ;  HETEROCYCLES ;  REAGENTS
语种: 英语
WOS记录号: WOS:000398985800081
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/150333
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
2.Dalian Univ Technol, Sch Chem & Chem Engn, Dalian 116023, Peoples R China
3.Univ Manchester, Sch Chem, Manchester M13 9PL, Lancs, England

Recommended Citation:
Wang, Fen,Jin, Liang,Kong, Lingheng,et al. Cobalt(III)- and Rhodium(III)-Catalyzed C-H Amidation and Synthesis of 4-Quinolones: C-H Activation Assisted by Weakly Coordinating and Functionalizable Enaminone[J]. ORGANIC LETTERS,2017,19(7):1812-1815.
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