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题名: Ruthenium-Catalyzed [3+2] Cycloaddition of 2H-Azirines with Alkynes: Access to Polysubstituted Pyrroles
作者: Li, Tengfei1, 2;  Yan, Hao1, 2;  Li, Xincheng1;  Wang, Chunxiang1;  Wan, Boshun1
刊名: JOURNAL OF ORGANIC CHEMISTRY
发表日期: 2016-12-02
DOI: 10.1021/acs.joc.6b02322
卷: 81, 期:23, 页:12031-12037
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Organic
英文摘要: A ruthenium-catalyzed intermolecular [3 + 2] cycloaddition of 2H-azirines and activated alkynes is reported, which provides polysubstituted pyrroles in moderate to good yields. This approach features a C-N bond cleavage of 2H-azirines by a ruthenium catalyst. The results of this study would provide a complementary method to synthesize polysubstituted pyrroles from the known 2H-azirine approaches and advance 2H-azirine chemistry.
关键词[WOS]: DIAZO OXIME ETHERS ;  C BOND-CLEAVAGE ;  STEREOSELECTIVE-SYNTHESIS ;  MULTICOMPONENT REACTIONS ;  SUBSTITUTED PYRROLES ;  AEROBIC SYNTHESIS ;  PYRIDINES ;  DIYNES ;  CYCLIZATION ;  CHEMISTRY
语种: 英语
WOS记录号: WOS:000389396400055
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/150422
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, 457 Zhongshan Rd, Dalian 116023, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China

Recommended Citation:
Li, Tengfei,Yan, Hao,Li, Xincheng,et al. Ruthenium-Catalyzed [3+2] Cycloaddition of 2H-Azirines with Alkynes: Access to Polysubstituted Pyrroles[J]. JOURNAL OF ORGANIC CHEMISTRY,2016,81(23):12031-12037.
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