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Adsorption/reaction energetics measured by microcalorimetry and correlated with reactivity on supported catalysts: A review
Li, Lin1; Lin, Jian1; Li, Xiaoyu1,2; Wang, Aiqin1; Wang, Xiaodong1; Zhang, Tao1
关键词Catalysis Microcalorimetry Reactivity Energetics Binding Strength Catalyst Characterization
刊名CHINESE JOURNAL OF CATALYSIS
2016-12-01
DOI10.1016/S1872-2067(16)62578-0
37期:12页:2039-2052
收录类别SCI
文章类型Review
WOS标题词Science & Technology ; Physical Sciences ; Technology
类目[WOS]Chemistry, Applied ; Chemistry, Physical ; Engineering, Chemical
研究领域[WOS]Chemistry ; Engineering
关键词[WOS]ACID-BASE PROPERTIES ; POLYCRYSTALLINE GOLD CATALYSTS ; TEMPERATURE CO OXIDATION ; N-BUTANE ISOMERIZATION ; GAS-PHASE DEHYDRATION ; SULFATED ZIRCONIA ; NICKEL-CATALYSTS ; ISOBUTANE DEHYDROGENATION ; HETEROGENEOUS CATALYSIS ; TUNGSTATED ZIRCONIA
英文摘要The formations and transformations of the chemical bonds of reactants and intermediates on catalyst surfaces occur in conjunction with the evolution of heat during catalytic reactions. Measurement of this evolved heat is helpful in terms of understanding the nature of the interactions between the catalyst and the adsorbed species, and provides insights into the reactivity of the catalyst. Although various techniques have previously been applied to assessments of evolved heat, direct measurements using a Tian-Calvet microcalorimeter are currently the most reliable method for this purpose. In this review, we summarize the relationship between the adsorption/reaction energetics determined by microcalorimetry and the reactivrties of supported catalysts, and examine the important role of microcalorimetry in understanding catalytic performance from the energetic point of view. (C) 2016, Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. All rights reserved.
语种英语
WOS记录号WOS:000391777500001
引用统计
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/151860
专题中国科学院大连化学物理研究所
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Liaoning, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
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GB/T 7714
Li, Lin,Lin, Jian,Li, Xiaoyu,et al. Adsorption/reaction energetics measured by microcalorimetry and correlated with reactivity on supported catalysts: A review[J]. CHINESE JOURNAL OF CATALYSIS,2016,37(12):2039-2052.
APA Li, Lin,Lin, Jian,Li, Xiaoyu,Wang, Aiqin,Wang, Xiaodong,&Zhang, Tao.(2016).Adsorption/reaction energetics measured by microcalorimetry and correlated with reactivity on supported catalysts: A review.CHINESE JOURNAL OF CATALYSIS,37(12),2039-2052.
MLA Li, Lin,et al."Adsorption/reaction energetics measured by microcalorimetry and correlated with reactivity on supported catalysts: A review".CHINESE JOURNAL OF CATALYSIS 37.12(2016):2039-2052.
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