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Numerical investigation on CO2 absorbed in aqueous N-methyldiethanolamine plus piperazine
Huang, Jicai1,2; Gong, Maoqiong1; Sun, Zhaohu1; Dong, Xueqiang1; Shen, Jun1; Wu, Jianfeng1
关键词Chemical Absorption Computational Fluid Dynamics Carbon Dioxide N-methyldiethanolamine Piperazine
刊名AICHE JOURNAL
2017-06-01
DOI10.1002/aic.15590
63期:6页:2386-2393
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Technology
类目[WOS]Engineering, Chemical
研究领域[WOS]Engineering
关键词[WOS]INSTANTANEOUS CHEMICAL-REACTION ; LAMINAR FALLING FILM ; PHASE MASS-TRANSFER ; GAS LOADING REGION ; CARBON-DIOXIDE ; ENHANCEMENT FACTORS ; ABSORPTION ; LIQUID ; SOLUBILITY ; FLOW
英文摘要A multiphase and multicomponent mass transfer model of CO2 absorbed in aqueous N-methyldiethanolamine and piperazine (PZ) was built in the study. In the model, a simple method of mass transfer between phases was proposed. Besides, the hydrodynamics, thermodynamics, and complex reversible chemical reaction were considered simultaneously. The model was validated by comparing with the previous experimental data which showed that simulated results can represent the experimental data with reasonable accuracy. Based on the model, the effects of gas velocity, liquid load and CO2 loading on the absorption rate, and enhancement factor were analyzed. Model results showed that the enhancement factor increased with a rising gas velocity while decreased with a rising liquid load or CO2 loading. The change of enhancement factor with CO2 loading was similar to that of equilibrium concentration of PZ which indicated that PZ was significant to the absorption process. Furthermore, the distributions of specie concentrations were discussed in detail. (c) 2016 American Institute of Chemical Engineers AIChE J, 63: 2386-2393, 2017
语种英语
WOS记录号WOS:000400658400051
引用统计
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/151971
专题中国科学院大连化学物理研究所
作者单位1.Chinese Acad Sci, Tech Inst Phys & Chem, Key Lab Cryogen, Beijing 100190, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, Div Fuel Cell & Battery, Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China
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GB/T 7714
Huang, Jicai,Gong, Maoqiong,Sun, Zhaohu,et al. Numerical investigation on CO2 absorbed in aqueous N-methyldiethanolamine plus piperazine[J]. AICHE JOURNAL,2017,63(6):2386-2393.
APA Huang, Jicai,Gong, Maoqiong,Sun, Zhaohu,Dong, Xueqiang,Shen, Jun,&Wu, Jianfeng.(2017).Numerical investigation on CO2 absorbed in aqueous N-methyldiethanolamine plus piperazine.AICHE JOURNAL,63(6),2386-2393.
MLA Huang, Jicai,et al."Numerical investigation on CO2 absorbed in aqueous N-methyldiethanolamine plus piperazine".AICHE JOURNAL 63.6(2017):2386-2393.
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